Flexible breathable photothermal-therapy epidermic sensor with MXene for ultrasensitive wearable human-machine interaction

被引:126
作者
Chao, Mingyuan [1 ]
Di, Pengju [1 ]
Yuan, Yue [1 ]
Xu, Yajin [1 ]
Zhang, Liqun [1 ]
Wan, Pengbo [1 ]
机构
[1] Beijing Univ Chem Technol, Coll Mat Sci & Engn, Interdisciplinary Res Ctr Artificial Intelligence, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
基金
中国国家自然科学基金; 北京市自然科学基金;
关键词
Flexible breathable epidermic sensor; Photothermal therapy; MXene; Ultrasensitive wearable human-machine interaction; Electronic skin; STRAIN SENSOR;
D O I
10.1016/j.nanoen.2023.108201
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Multifunctional flexible wearable epidermic sensors have gained enormous attention for their promising potential applications in personal health management, electronic skins and intelligent human-machine interaction. However, it remains a critical challenge to realize a flexible breathable sensing device with reliable sensing performances for comfortably wearable human motion detection and ultrasensitive human-machine interfacing with the integrated functional capability of disease diagnosis and subsequent photothermal therapy simultaneously. Herein, a flexible breathable epidermic sensor is fabricated by delicately assembling conductive MXene nanosheets and silver nanowires (AgNWs) onto electrospun elastomeric substrates for ultrasensitive sensing and on-demand photothermal therapy. The as-prepared flexible breathable electronic sensor presents a broad sensing range (up to similar to 120 %), ultrahigh sensitivity (gauge factor (GF) up to 4720), extremely low detection limit, remarkable reliability, and robust biocompatibility for serving as the electronic skin to monitor human physiological signals and wearable human-machine interaction. Moreover, it exhibits brilliant photothermal properties for enhanced antibacterial effect and timely photothermal therapy after healthcare monitoring and disease diagnosis. This work provides a facile way of developing flexible breathable multifunctional electronic sensors featured with excellent sensing ability, brilliant breathability and reliable photothermal properties for long-term healthcare monitoring, ultrasensitive wearable human-machine interfacing, smart disease diagnosis and treatment.
引用
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页数:10
相关论文
共 55 条
[1]   Highly Stretchable and Sensitive Strain Sensor Based on Silver Nanowire-Elastomer Nanocomposite [J].
Amjadi, Morteza ;
Pichitpajongkit, Aekachan ;
Lee, Sangjun ;
Ryu, Seunghwa ;
Park, Inkyu .
ACS NANO, 2014, 8 (05) :5154-5163
[2]   MXene-Reinforced Cellulose Nanofibril Inks for 3D-Printed Smart Fibres and Textiles [J].
Cao, Wen-Tao ;
Ma, Chang ;
Mao, Dong-Sheng ;
Zhang, Juan ;
Ma, Ming-Guo ;
Chen, Feng .
ADVANCED FUNCTIONAL MATERIALS, 2019, 29 (51)
[3]   Breathable Ti3C2Tx MXene/Protein Nanocomposites for Ultrasensitive Medical Pressure Sensor with Degradability in Solvents [J].
Chao, Mingyuan ;
He, Lingzhang ;
Gong, Min ;
Li, Na ;
Li, Xiaobin ;
Peng, Longfei ;
Shi, Feng ;
Zhang, Liqun ;
Wan, Pengbo .
ACS NANO, 2021, 15 (06) :9746-9758
[4]   Wearable MXene nanocomposites-based strain sensor with tile-like stacked hierarchical microstructure for broad-range ultrasensitive sensing [J].
Chao, Mingyuan ;
Wang, Yonggang ;
Ma, Di ;
Wu, Xiaoxuan ;
Zhang, Weixia ;
Zhang, Liqun ;
Wan, Pengbo .
NANO ENERGY, 2020, 78
[5]   Hierarchical elastomer tuned self-powered pressure sensor for wearable multifunctional cardiovascular electronics [J].
Chen, Shuwen ;
Wu, Nan ;
Lin, Shizhe ;
Duan, Jiangjiang ;
Xu, Zisheng ;
Pan, Yuan ;
Zhang, Hongbo ;
Xu, Zheheng ;
Huang, Liang ;
Hu, Bin ;
Zhou, Jun .
NANO ENERGY, 2020, 70
[6]   Bioinspired Microspines for a High-Performance Spray Ti3C2Tx MXene-Based Piezoresistive Sensor [J].
Cheng, Yongfa ;
Ma, Yanan ;
Li, Luying ;
Zhu, Meng ;
Yue, Yang ;
Liu, Weijie ;
Wang, Longfei ;
Jia, Shuangfeng ;
Li, Chen ;
Qi, Tianyu ;
Wang, Jianbo ;
Gao, Yihua .
ACS NANO, 2020, 14 (02) :2145-2155
[7]   Stretchable Heater Using Ligand-Exchanged Silver Nanowire Nanocomposite for Wearable Articular Thermotherapy [J].
Choi, Suji ;
Park, Jinkyung ;
Hyun, Wonji ;
Kim, Jangwon ;
Kim, Jaemin ;
Lee, Young Bum ;
Song, Changyeong ;
Hwang, Hye Jin ;
Kim, Ji Hoon ;
Hyeon, Taeghwan ;
Kim, Dae-Hyeong .
ACS NANO, 2015, 9 (06) :6626-6633
[8]   A Wearable Transient Pressure Sensor Made with MXene Nanosheets for Sensitive Broad-Range Human-Machine Interfacing [J].
Guo, Ying ;
Zhong, Mengjuan ;
Fang, Zhiwei ;
Wan, Pengbo ;
Yu, Guihua .
NANO LETTERS, 2019, 19 (02) :1143-1150
[9]   Emerging 2D MXenes for supercapacitors: status, challenges and prospects [J].
Hu, Minmin ;
Zhang, Hui ;
Hu, Tao ;
Fan, Bingbing ;
Wang, Xiaohui ;
Li, Zhenjiang .
CHEMICAL SOCIETY REVIEWS, 2020, 49 (18) :6666-6693
[10]   2D MXenes for Electromagnetic Shielding: A Review [J].
Iqbal, Aamir ;
Sambyal, Pradeep ;
Koo, Chong Min .
ADVANCED FUNCTIONAL MATERIALS, 2020, 30 (47)