Opposite atom dependence of isotope engineering of thermal conductivity in bulk and 2D GaN

被引:1
作者
Sun, Guoqing [1 ]
Xiang, Zheng [1 ]
Ma, Jinlong [1 ]
Luo, Xiaobing [1 ]
Xu, Dongwei [1 ]
机构
[1] Huazhong Univ Sci & Technol, Sch Energy & Power Engn, State Key Lab Coal Combust, Wuhan, Peoples R China
基金
中国国家自然科学基金;
关键词
GaN; thermal conductivity; scattering rate; isotope engineering; TRANSPORT;
D O I
10.1088/1361-6528/acf503
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Isotope engineering has been shown to be an effective means of regulating thermal conductivity. In this work, we studied the isotope engineering of thermal conductivity in bulk and 2D GaN, and diametrically opposite atom isotope dependence is found. That is, Ga isotope has a large effect (77%) on bulk GaN, while the effect of N isotope on the thermal conductivity is negligible. In 2D GaN, however, N isotope effect (20%) is more significant than that of Ga. Understanding of the different isotope dependence is achieved by deeper insight. Due to the relative magnitude of scattering rate, isotopic scattering influences the thermal conductivity of bulk and 2D GaN in different frequency regions, leading to the opposite atom dependence.
引用
收藏
页数:6
相关论文
共 26 条
[1]   Outstanding Thermal Conductivity of Single Atomic Layer Isotope-Modified Boron Nitride [J].
Cai, Qiran ;
Scullion, Declan ;
Gan, Wei ;
Falin, Alexey ;
Cizek, Pavel ;
Liu, Song ;
Edgar, James H. ;
Liu, Rong ;
Li, Lu Hua ;
Cowie, Bruce C. C. ;
Santos, Elton J. G. .
PHYSICAL REVIEW LETTERS, 2020, 125 (08)
[2]   Ultrahigh thermal conductivity in isotope-enriched cubic boron nitride [J].
Chen, Ke ;
Song, Bai ;
Ravichandran, Navaneetha K. ;
Zheng, Qiye ;
Chen, Xi ;
Lee, Hwijong ;
Sun, Haoran ;
Li, Sheng ;
Gamage, Geethal Amila Udalamatta Gamage ;
Tian, Fei ;
Ding, Zhiwei ;
Song, Qichen ;
Rai, Akash ;
Wu, Hanlin ;
Koirala, Pawan ;
Schmidt, Aaron J. ;
Watanabe, Kenji ;
Lv, Bing ;
Ren, Zhifeng ;
Shi, Li ;
Cahill, David G. ;
Taniguchi, Takashi ;
Broido, David ;
Chen, Gang .
SCIENCE, 2020, 367 (6477) :555-+
[3]  
Chen SS, 2012, NAT MATER, V11, P203, DOI [10.1038/nmat3207, 10.1038/NMAT3207]
[4]   Thermal effect of epilayer on phonon transport of semiconducting heterostructure interfaces [J].
Huang, Xu ;
Guo, Zhixiong .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2021, 178
[5]   Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set [J].
Kresse, G ;
Furthmuller, J .
PHYSICAL REVIEW B, 1996, 54 (16) :11169-11186
[6]   ShengBTE: A solver of the Boltzmann transport equation for phonons [J].
Li, Wu ;
Carrete, Jesus ;
Katcho, Nebil A. ;
Mingo, Natalio .
COMPUTER PHYSICS COMMUNICATIONS, 2014, 185 (06) :1747-1758
[7]   Isotope-Engineering the Thermal Conductivity of Two-Dimensional MoS2 [J].
Li, Xufan ;
Zhang, Jingjie ;
Puretzky, Alexander A. ;
Yoshimura, Anthony ;
Sang, Xiahan ;
Cui, Qiannan ;
Li, Yuanyuan ;
Liang, Liangbo ;
Ghosh, Avik W. ;
Zhao, Hui ;
Unocic, Raymond R. ;
Meunier, Vincent ;
Rouleau, Christopher M. ;
Sumpter, Bobby G. ;
Geohegan, David B. ;
Xiao, Kai .
ACS NANO, 2019, 13 (02) :2481-2489
[8]   Phonon-isotope scattering and thermal conductivity in materials with a large isotope effect: A first-principles study [J].
Lindsay, L. ;
Broido, D. A. ;
Reinecke, T. L. .
PHYSICAL REVIEW B, 2013, 88 (14)
[9]   Thermal Conductivity and Large Isotope Effect in GaN from First Principles [J].
Lindsay, L. ;
Broido, D. A. ;
Reinecke, T. L. .
PHYSICAL REVIEW LETTERS, 2012, 109 (09)
[10]   Enhanced thermal conductivity and isotope effect in single-layer hexagonal boron nitride [J].
Lindsay, L. ;
Broido, D. A. .
PHYSICAL REVIEW B, 2011, 84 (15)