Enhancement of high-order harmonic generation in graphene by mid-infrared and terahertz fields

被引:1
作者
Mao, Wenwen [1 ]
Rubio, Angel [1 ,2 ]
Sato, Shunsuke A. [1 ,3 ]
机构
[1] Max Planck Inst Struct & Dynam Matter, Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany
[2] Flatiron Inst, Ctr Computat Quantum Phys, New York, NY 10010 USA
[3] Univ Tsukuba, Ctr Computat Sci, Tsukuba 3058577, Japan
关键词
RADIATION; ELECTRONS; DYNAMICS; STATES;
D O I
10.1103/PhysRevB.109.045421
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We theoretically investigate high-order harmonic generation (HHG) in graphene under mid-infrared (MIR) and terahertz (THz) fields based on a quantum master equation. Numerical simulations show that MIR-induced HHG in graphene can be enhanced by a factor of 10 for fifth harmonic and a factor of 25 for seventh harmonic under a THz field with a peak strength of 0.5 MV/cm by optimizing the relative angle between the MIR and THz fields. To identify the origin of this enhancement, we compare the fully dynamical calculations with a simple thermodynamic model and a nonequilibrium population model. The analysis shows that the enhancement of the high-order harmonics mainly results from a coherent coupling between MIR- and THz-induced transitions that goes beyond a simple THz-induced population contribution.
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页数:12
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