Experimental study of the removal NOx and SO2 from flue gas using the O3/H2O2, and O3/UV processes

被引:2
|
作者
Dalal, Parveen [1 ]
Dalai, Sridhar [1 ]
Khuntia, Snigdha [1 ]
机构
[1] Ahmedabad Univ, Sch Engn & Appl Sci, Ahmadabad 380009, Gujarat, India
关键词
Energy calculation; flue gas; hydroxyl radicals; ozonation; UV intensity; NITRIC-OXIDE; PHOTOCHEMICAL OXIDATION; PHOTO-FENTON; ABSORPTION; ULTRAVIOLET; KINETICS; UV-H2O2; OZONE; WATER;
D O I
10.1080/09593330.2023.2256991
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The study investigates the effect of different parameters for the removal of SO2 and NOx through a wet process concurrently. Two separate processes have been compared for the removal of flue gases, that is, Ozone/UV and H2O2/UV. The research aims to develop a comparative study for the removal of SO2 and NOx simultaneously using Ozone/H2O2 and UV light and find the energy consumption (also known as E-EO) for each process. Combining UV with O-3 and H2O2 play a crucial role in generating hydroxyl radicals. Different combinations of Ozone/H2O2, flue gas, and UV intensity were studied at different pH and temperatures of the solution to achieve maximum removal of the flue gases. For, the ozonation process it was observed that the removal% of flue gases increases with increasing UV intensity, and at higher UV intensity (250 W), the removal% for NOx is 92% and SO2 is 95% simultaneously at optimum temperature 308 K. For H2O2/UV process (250 W UV intensity), removal% for NOx is 95% and SO2 is 100% at 313 K, 0.3 LPM flow rate of flue gases. The E-EO values obtained for both processes were less than 1 for 95% NOx/SO2 removal efficiency.
引用
收藏
页码:4526 / 4535
页数:10
相关论文
共 50 条
  • [11] Decolorization and Modeling of Synthetic Wastewater Using O3 and H2O2/O3 Processes
    Bauman, M.
    Lobnik, A.
    Hribernik, A.
    OZONE-SCIENCE & ENGINEERING, 2011, 33 (01) : 23 - 30
  • [12] Degradation performance and conversion mechanisms of MNZ by advanced oxidation systems with O3: Comparison of O3, O3/UV, O3/H2O2 and UV-H2O2/O3 systems
    Ren, Yuehua
    Wang, Yonglei
    Xue, Jie
    Liu, Baozhen
    He, Guilin
    Jia, Weijian
    Liu, Baosen
    Jia, Ruibao
    JOURNAL OF WATER PROCESS ENGINEERING, 2024, 68
  • [13] A quantum chemistry study on reaction mechanisms of SO2 with O3 and H2O2
    Jiang, Shu-dong
    Wang, Zhi-hua
    Zhou, Jun-hu
    Wen, Zheng-cheng
    Cen, Ke-fa
    JOURNAL OF ZHEJIANG UNIVERSITY-SCIENCE A, 2009, 10 (09): : 1327 - 1333
  • [15] A quantum chemistry study on reaction mechanisms of SO2 with O3 and H2O2
    Shu-dong Jiang
    Zhi-hua Wang
    Jun-hu Zhou
    Zheng-cheng Wen
    Ke-fa Cen
    Journal of Zhejiang University-SCIENCE A, 2009, 10 : 1327 - 1333
  • [16] Simultaneous Removal of NO and SO2 from Flue Gas by UV/H2O2/CaO
    Liu, Yangxian
    Zhang, Jun
    Wang, Zhuliang
    Du, Min
    CHEMICAL ENGINEERING & TECHNOLOGY, 2012, 35 (10) : 1879 - 1884
  • [17] Use of response surface methodology for pretreatment of hospital wastewater by O3/UV and O3/UV/H2O2 processes
    Arslan, Ayla
    Veli, Sevil
    Bingol, Deniz
    SEPARATION AND PURIFICATION TECHNOLOGY, 2014, 132 : 561 - 567
  • [18] Simazine removal from water in a continuous bubble column by O3 and O3/H2O2
    Rivas, J
    Beltrán, FJ
    García-Araya, JF
    Navarrete, V
    JOURNAL OF ENVIRONMENTAL SCIENCE AND HEALTH PART B-PESTICIDES FOOD CONTAMINANTS AND AGRICULTURAL WASTES, 2001, 36 (06) : 809 - 819
  • [19] ACIDIFICATION OF RAIN IN THE PRESENCE OF SO2, H2O2, O3 AND HNO3
    DURHAM, JL
    OVERTON, JH
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1981, 181 (MAR): : 58 - ENVR
  • [20] Comparison of sludge treatment by O3 and O3/H2O2
    Zhao Yuxin
    Wang Liang
    Yu Helong
    Jiang Baojun
    Jiang Jinming
    WATER SCIENCE AND TECHNOLOGY, 2014, 70 (01) : 114 - 119