Electrospinning CeO2/g-C3N4 Nanofibers for Efficient Photocatalytic Degradation Performance

被引:1
作者
Du, Ping [1 ]
Duan, Yongzheng [1 ]
Shang, Xili [1 ]
机构
[1] Binzhou Univ, Dept Chem Engn & Safety, Binzhou 256600, Shandong, Peoples R China
关键词
CeO2; g-C3N4; electrospinning nanofiber; photocatalytic activity; IN-SITU FABRICATION; COMPOSITE; HETEROJUNCTION; TETRACYCLINE; NANOSHEETS;
D O I
10.1134/S0036024423010259
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A serials of nanofibers with different contents of CeO2 were successfully fabricated by electrospinning techniques. The structure, morphology and optical properties were characterized by X-ray diffraction, Scanning electron microscopy, Fourier transform infrared spectra, X-ray photoelectron spectroscopy, UV-Vis spectroscopy. The catalytic properties of CeO2/g-C3N4 composites were evaluated using tetracycline hydrochloride under simulated solar light illumination. When the loading amount of CeO2 was 5.0 wt %, the composite showed the highest catalytic activity, which was 5.8 times that of porous g-C3N4. The enhanced photocatalytic properties of CeO2/g-C3N4 may be attributed to effective separation of photogenerated carriers and enhanced absorption of visible light. The photocatalyst had an excellent catalytic stability and possible photodegradation mechanism of the obtained sample was proposed.
引用
收藏
页码:293 / 298
页数:6
相关论文
共 32 条
[1]   Enhanced catalytic degradation of AO7 in the CeO2-H2O2 system with Fe3+ doping [J].
Cai, Wandong ;
Chen, Feng ;
Shen, Xingxing ;
Chen, Lijing ;
Zhang, Jinlong .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2010, 101 (1-2) :160-168
[2]   The Role of Polarization in Photocatalysis [J].
Chen, Fang ;
Huang, Hongwei ;
Guo, Lin ;
Zhang, Yihe ;
Ma, Tianyi .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2019, 58 (30) :10061-10073
[3]   Efficient synthesis of polymeric g-C3N4 layered materials as novel efficient visible light driven photocatalysts [J].
Dong, Fan ;
Wu, Liwen ;
Sun, Yanjuan ;
Fu, Min ;
Wu, Zhongbiao ;
Lee, S. C. .
JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (39) :15171-15174
[4]   Direct Z-scheme Bi2O2CO3/porous g-C3N4 heterojunction for improved photocatalytic degradation performance [J].
Duan, Yongzheng ;
Li, Jing ;
Li, Yuejin ;
Shang, Xili ;
Jia, Dongmei ;
Li, Changhai .
JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS, 2020, 106 :74-85
[5]   Improved Solar-Driven Photocatalytic Activity of Hybrid Graphene Quantum Dots/ZnO Nanowires: A Direct Z-Scheme Mechanism [J].
Ebrahimi, Mandi ;
Samadi, Morasae ;
Yousefzadeh, Samira ;
Soltani, Mojtaba ;
Rahimi, Alireza ;
Chou, Tsu-chin ;
Chen, Li-Chyong ;
Chen, Kuei-Hsien ;
Moshfegh, Alireza Zaker .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2017, 5 (01) :367-375
[6]   In situ synthesis of graphitic-C3N4 nanosheet hybridized N-doped TiO2 nanofibers for efficient photocatalytic H2 production and degradation [J].
Han, Cheng ;
Wang, Yingde ;
Lei, Yongpeng ;
Wang, Bing ;
Wu, Nan ;
Shi, Qi ;
Li, Qiong .
NANO RESEARCH, 2015, 8 (04) :1199-1209
[7]   Room-temperature in situ fabrication and enhanced photocatalytic activity of direct Z-scheme BiOI/g-C3N4 photocatalyst [J].
He, Rongan ;
Cheng, Kaiyu ;
Wei, Zheying ;
Zhang, Shiying ;
Xu, Difa .
APPLIED SURFACE SCIENCE, 2019, 465 :964-972
[8]   Room-temperature in situ fabrication of Bi2O3/g-C3N4 direct Z-scheme photocatalyst with enhanced photocatalytic activity [J].
He, Rongan ;
Zhou, Jiaqian ;
Fu, Huiqing ;
Zhang, Shiying ;
Jiang, Chuanjia .
APPLIED SURFACE SCIENCE, 2018, 430 :273-282
[9]   Macroscopic Polarization Enhancement Promoting Photo- and Piezoelectric-Induced Charge Separation and Molecular Oxygen Activation [J].
Huang, Hongwei ;
Tu, Shuchen ;
Zeng, Chao ;
Zhang, Tierui ;
Reshak, Ali H. ;
Zhang, Yihe .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (39) :11860-11864
[10]   In situ assembly of BiOI@Bi12O17Cl2 p-n junction: charge induced unique front-lateral surfaces coupling heterostructure with high exposure of BiOI {001} active facets for robust and nonselective photocatalysis [J].
Huang, Hongwei ;
Xiao, Ke ;
He, Ying ;
Zhang, Tierui ;
Dong, Fan ;
Du, Xin ;
Zhang, Yihe .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2016, 199 :75-86