Recycling of graphite anode from spent lithium-ion batteries: Advances and perspectives

被引：76

作者：

Qiao, Yu ^{[1
,2
]}

Zhao, Huaping ^{[2
]}

Shen, Yonglong ^{[3
]}

Li, Liqiang ^{[4
]}

Rao, Zhonghao ^{[1
]}

Shao, Guosheng ^{[3
]}

Lei, Yong ^{[2
]}

机构：

[1] Hebei Univ Technol, Sch Energy & Environm Engn, Hebei Key Lab Thermal Sci & Energy Clean Utilizat, Tianjin 300401, Peoples R China

[2] Tech Univ Ilmenau, Inst Phys & IMN MacroNano, Fachgebiet Angew Nanophys, Ilmenau, Germany

[3] Zhengzhou Univ, Sch Mat Sci & Engn, Zhengzhou 450001, Peoples R China

[4] Tianjin Univ, Inst Mol Aggregat Sci, Dept Chem, Tianjin Key Lab Mol Optoelect Sci, Tianjin, Peoples R China

来源：

ECOMAT | 2023年 / 5卷 / 04期

关键词：

graphite anode; recycling; regeneration; reutilization; spent lithium-ion batteries; SOLID-ELECTROLYTE INTERPHASE; REDUCED GRAPHENE OXIDE; IN-SITU; CATALYTIC PERFORMANCE; LITHIATED GRAPHITE; FAILURE MECHANISMS; CATHODE MATERIALS; DENDRITIC GROWTH; CRACK FORMATION; CURRENT-DENSITY;

D O I：

10.1002/eom2.12321

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

There is growing production for lithium-ion batteries (LIBs) to satisfy the booming development renewable energy storage systems. Meanwhile, amounts of spent LIBs have been generated and will become more soon. Therefore, the proper disposal of these spent LIBs is of significant importance. Graphite is the dominant anode in most commercial LIBs. This review specifically focuses on the recent advances in the recycling of graphite anode (GA) from spent LIBs. It covers the significance of GA recycling from spent LIBs, the introduction of the GA aging mechanisms in LIBs, the summary of the developed GA recovery strategies, and the highlight of reclaimed GA for potential applications. In addition, the prospect related to the future challenges of GA recycling is given at the end. It is expected that this review will provide practical guidance for researchers engaged in the field of spent LIBs recycling.

引用

页数：27

共 164 条

[81] Internal failure of anode materials for lithium batteries - A critical review [J].

Meng, Xiangqi ;

Xu, Yaolin ;

Cao, Hongbin ;

Lin, Xiao ;

Ning, Pengge ;

Zhang, Yi ;

Garcia, Yaiza Gonzalez ;

Sun, Zhi .

GREEN ENERGY & ENVIRONMENT, 2020, 5 (01) :22-36

[82] Recycling of graphite anodes for the next generation of lithium ion batteries [J].

Moradi, Bahar ;

Botte, Gerardine G. .

JOURNAL OF APPLIED ELECTROCHEMISTRY, 2016, 46 (02) :123-148

[83] Electrochemical behavior and passivation of current collectors in lithium-ion batteries [J].

Myung, Seung-Taek ;

Hitoshi, Yashiro ;

Sun, Yang-Kook .

JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (27) :9891-9911

[84] Should we recycle the graphite from spent lithium-ion batteries? The untold story of graphite with the importance of recycling [J].

Natarajan, Subramanian ;

Divya, Madhusoodhanan Lathika ;

Aravindan, Vanchiappan .

JOURNAL OF ENERGY CHEMISTRY, 2022, 71 :351-369

[85] Recycling/Reuse of Current Collectors from Spent Lithium-Ion Batteries: Benefits and Issues [J].

Natarajan, Subramanian ;

Akshay, Manohar ;

Aravindan, Vanchiappan .

ADVANCED SUSTAINABLE SYSTEMS, 2022, 6 (03)

[86] An Urgent Call to Spent LIB Recycling: Whys and Wherefores for Graphite Recovery [J].

Natarajan, Subramanian ;

Aravindan, Vanchiappan .

ADVANCED ENERGY MATERIALS, 2020, 10 (37)

[87] Template-free synthesis of carbon hollow spheres and reduced graphene oxide from spent lithium-ion batteries towards efficient gas storage [J].

Natarajan, Subramanian ;

Bajaj, Hari C. ;

Aravindan, Vanchiappan .

JOURNAL OF MATERIALS CHEMISTRY A, 2019, 7 (07) :3244-3252

[88] Environmental benign synthesis of reduced graphene oxide (rGO) from spent lithium-ion batteries (LIBs) graphite and its application in supercapacitor [J].

Natarajan, Subramanian ;

Ede, Sivasankara Rao ;

Bajaj, Hari C. ;

Kundu, Subrata .

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2018, 543 :98-108

[89] Recovery and utilization of graphite and polymer materials from spent lithium-ion batteries for synthesizing polymer-graphite nanocomposite thin films [J].

Natarajan, Subramanian ;

Lakshmi, D. Shanthana ;

Bajaj, Hari C. ;

Srivastava, Divesh N. .

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2015, 3 (04) :2538-2545

[90] Anode carbonaceous material recovered from spent lithium-ion batteries in electric vehicles for environmental application [J].

Nguyen, Thi-Hai Anh ;

Oh, Seok-Young .

WASTE MANAGEMENT, 2021, 120 :755-761

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