High-throughput screening of superior hydrogen evolution reaction catalysts in Pd-Ni-Fe alloys

被引:7
|
作者
Zou, Peng [1 ,2 ,3 ]
Song, Lijian [1 ,2 ,3 ]
Xu, Wei [1 ,2 ,3 ]
Gao, Meng [1 ,2 ,3 ]
Zadorozhnyy, Vladislav [4 ]
Huo, Juntao [1 ,2 ,3 ]
Wang, Jun-Qiang [1 ,2 ,3 ]
机构
[1] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, CAS Key Lab Magnet Mat & Devices, Ningbo 315201, Peoples R China
[2] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Zhejiang Prov Key Lab Magnet Mat & Applicat Techno, Ningbo 315201, Peoples R China
[3] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
[4] Natl Univ Sci & Technol MISIS, Leninsky Prosp 4, Moscow 119049, Russia
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
High-throughput strategy; Magnetron co-sputtering; Bubble screening; Electrocatalyst; Hydrogen evolution reaction; ELECTROCATALYTIC HYDROGEN; EFFICIENT; NANOCLUSTERS; ELECTRODE; BORIDE; CARBON; GLASS;
D O I
10.1016/j.jallcom.2023.170656
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The development of efficient multicomponent catalysts with high intrinsic catalytic activity is a critical challenge for hydrogen evolution reaction (HER). Herein, an efficient Pd-Ni-Fe HER catalyst is designed by using high-throughput bubble screening method. The Pd63Ni16Fe21 catalyst shows excellent HER perfor-mance in 0.5 M H2SO4 solution, which is preferable to the other Pd-based catalysts. The outstanding cat-alytic activity is attributed to the optimized alloy composition. The results demonstrate that high-throughput bubble screening is an effective method to discover multicomponent alloys with superior HER performance experimentally.(c) 2023 Elsevier B.V. All rights reserved.
引用
收藏
页数:8
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