Activated porous carbon sorbents;
N and O codoped atmosphere water harvesting;
Fast solar-driven desorption;
Heterogeneity;
Hierarchical porous structure;
METAL-ORGANIC FRAMEWORKS;
ADSORPTION;
HYDROPHILICITY;
GROWTH;
D O I:
10.1016/j.apmt.2024.102121
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
There is significant interest in developing high-performance adsorbents that can harvest water from atmospheric air powered by sunlight. However, The inherent hydrophobicity of porous carbon limits water harvesting capacity. Herein, we report a new class of activated porous carbons (PAK-21) with high water adsorption capacity at moderate to high humidity by solid-phase polymerization of terephthalaldehyde and 2,6-diaminopurine in the presence of KOH under an argon atmosphere at 150 degrees C for 2 h, and then activated at a high temperature of 700 degrees C for 1 h. The water harvesting performance surpasses the most common MOFs and porous carbon adsorbents, which benefit from rich surface heterogeneity and highly porous structure. PAK-21 also exhibits fast solar-driven desorption kinetics, ascribing to rapid photothermal responsiveness, hierarchical porosity, and suitable hydrophilicity. Besides, twenty-one adsorption-desorption cycles have been performed to demonstrate its easy regeneration and long-term cyclability. This may pave a new way to modulate the surface functionality and microporous/mesoporous engineering of carbon adsorbents for high-performance solar-driven AWH.
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Bai, Jiali
Huang, Jiamei
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Huang, Jiamei
Yu, Qiyun
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Yu, Qiyun
论文数: 引用数:
h-index:
机构:
Demir, Muslum
Akgul, Eda
论文数: 0引用数: 0
h-index: 0
机构:
Osmaniye Korkut Ata Univ, Dept Chem Engn, TR-80000 Osmaniye, TurkiyeZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Akgul, Eda
Altay, Bilge Nazli
论文数: 0引用数: 0
h-index: 0
机构:
Rochester Inst Technol, Coll Engn Technol Print & Graph Media Sci, New York, NY 14623 USA
Marmara Univ, Inst Pure & Appl Sci, TR-34722 Istanbul, TurkiyeZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Altay, Bilge Nazli
Hu, Xin
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Hu, Xin
Wang, Linlin
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Coll Engn, Key Lab Urban Rail Transit Intelligent Operat & Ma, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
机构:
Tokyo Univ Agr & Technol, Grad Sch Engn, 2-24-16 Naka Cho, Koganei, Tokyo 1848588, Japan
Res Inst Innovat Technol Earth RITE, Chem Res Grp, 9-2 Kizugawadai, Kizugawa, Kyoto 6190292, JapanTokyo Univ Agr & Technol, Grad Sch Engn, 2-24-16 Naka Cho, Koganei, Tokyo 1848588, Japan
Fujiki, Junpei
Yogo, Katsunori
论文数: 0引用数: 0
h-index: 0
机构:
Res Inst Innovat Technol Earth RITE, Chem Res Grp, 9-2 Kizugawadai, Kizugawa, Kyoto 6190292, JapanTokyo Univ Agr & Technol, Grad Sch Engn, 2-24-16 Naka Cho, Koganei, Tokyo 1848588, Japan
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Hanikel, Nikita
Pei, Xiaokun
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Pei, Xiaokun
论文数: 引用数:
h-index:
机构:
Chheda, Saumil
Lyu, Hao
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Lyu, Hao
Jeong, WooSeok
论文数: 0引用数: 0
h-index: 0
机构:
Univ Minnesota, Minnesota Supercomp Inst, Minneapolis, MN 55455 USA
Univ Minnesota, Chem Theory Ctr, Dept Chem, Minneapolis, MN 55455 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Jeong, WooSeok
Sauer, Joachim
论文数: 0引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Chem, D-10099 Berlin, GermanyUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Sauer, Joachim
Gagliardi, Laura
论文数: 0引用数: 0
h-index: 0
机构:
Univ Chicago, Dept Chem, Pritzker Sch Mol Engn, James Franck Inst, Chicago, IL 60637 USA
Univ Chicago, Chicago Ctr Theoret Chem, Chicago, IL 60637 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Gagliardi, Laura
Yaghi, Omar M.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Bai, Jiali
Huang, Jiamei
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Huang, Jiamei
Yu, Qiyun
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Yu, Qiyun
论文数: 引用数:
h-index:
机构:
Demir, Muslum
Akgul, Eda
论文数: 0引用数: 0
h-index: 0
机构:
Osmaniye Korkut Ata Univ, Dept Chem Engn, TR-80000 Osmaniye, TurkiyeZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Akgul, Eda
Altay, Bilge Nazli
论文数: 0引用数: 0
h-index: 0
机构:
Rochester Inst Technol, Coll Engn Technol Print & Graph Media Sci, New York, NY 14623 USA
Marmara Univ, Inst Pure & Appl Sci, TR-34722 Istanbul, TurkiyeZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Altay, Bilge Nazli
Hu, Xin
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
Hu, Xin
Wang, Linlin
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Normal Univ, Coll Engn, Key Lab Urban Rail Transit Intelligent Operat & Ma, Jinhua 321004, Peoples R ChinaZhejiang Normal Univ, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
机构:
Tokyo Univ Agr & Technol, Grad Sch Engn, 2-24-16 Naka Cho, Koganei, Tokyo 1848588, Japan
Res Inst Innovat Technol Earth RITE, Chem Res Grp, 9-2 Kizugawadai, Kizugawa, Kyoto 6190292, JapanTokyo Univ Agr & Technol, Grad Sch Engn, 2-24-16 Naka Cho, Koganei, Tokyo 1848588, Japan
Fujiki, Junpei
Yogo, Katsunori
论文数: 0引用数: 0
h-index: 0
机构:
Res Inst Innovat Technol Earth RITE, Chem Res Grp, 9-2 Kizugawadai, Kizugawa, Kyoto 6190292, JapanTokyo Univ Agr & Technol, Grad Sch Engn, 2-24-16 Naka Cho, Koganei, Tokyo 1848588, Japan
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Hanikel, Nikita
Pei, Xiaokun
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Pei, Xiaokun
论文数: 引用数:
h-index:
机构:
Chheda, Saumil
Lyu, Hao
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Lyu, Hao
Jeong, WooSeok
论文数: 0引用数: 0
h-index: 0
机构:
Univ Minnesota, Minnesota Supercomp Inst, Minneapolis, MN 55455 USA
Univ Minnesota, Chem Theory Ctr, Dept Chem, Minneapolis, MN 55455 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Jeong, WooSeok
Sauer, Joachim
论文数: 0引用数: 0
h-index: 0
机构:
Humboldt Univ, Inst Chem, D-10099 Berlin, GermanyUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Sauer, Joachim
Gagliardi, Laura
论文数: 0引用数: 0
h-index: 0
机构:
Univ Chicago, Dept Chem, Pritzker Sch Mol Engn, James Franck Inst, Chicago, IL 60637 USA
Univ Chicago, Chicago Ctr Theoret Chem, Chicago, IL 60637 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Gagliardi, Laura
Yaghi, Omar M.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USAUniv Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA