Wood-based superblack

被引:20
|
作者
Zhao, Bin [1 ]
Shi, Xuetong [2 ]
Khakalo, Sergei [3 ,4 ]
Meng, Yang [5 ]
Miettinen, Arttu [6 ]
Turpeinen, Tuomas [7 ]
Mi, Shuyi [8 ]
Sun, Zhipei [8 ,9 ]
Khakalo, Alexey [10 ]
Rojas, Orlando J. [1 ,2 ]
Mattos, Bruno D. [1 ]
机构
[1] Aalto Univ, Sch Chem Engn, Dept Bioprod & Biosyst, FI-02150 Espoo, Finland
[2] Univ British Columbia, Bioprod Inst, Vancouver, BC V6T 1Z3, Canada
[3] Aalto Univ, Sch Engn, Dept Civil Engn, FI-02150 Espoo, Finland
[4] VTT Tech Res Ctr Finland Ltd, Integrated Comp Mat Engn, FI-02044 Espoo, Finland
[5] Kunming Univ Sci & Technol, Fac Chem Engn, Kunming 650500, Peoples R China
[6] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland
[7] VTT Tech Res Ctr Finland Ltd, Fiber Web Proc, FI-40400 Jyvaskyla, Finland
[8] Aalto Univ, Dept Elect & Nanoengn, FI-02150 Espoo, Finland
[9] Aalto Univ, Dept Appl Phys, QTF Ctr Excellence, FI-02150 Espoo, Finland
[10] VTT Tech Res Ctr Finland Ltd, Cellulose Coatings & Films, FI-02044 Espoo, Finland
基金
欧盟地平线“2020”; 芬兰科学院; 加拿大创新基金会;
关键词
ALIGNED CARBON NANOTUBES; REFLECTANCE; ABSORBERS; SURFACES; AEROGELS;
D O I
10.1038/s41467-023-43594-4
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Light is a powerful and sustainable resource, but it can be detrimental to the performance and longevity of optical devices. Materials with near-zero light reflectance, i.e. superblack materials, are sought to improve the performance of several light-centered technologies. Here we report a simple top-down strategy, guided by computational methods, to develop robust superblack materials following metal-free wood delignification and carbonization (1500 degrees C). Subwavelength severed cells evolve under shrinkage stresses, yielding vertically aligned carbonmicrofiber arrayswith a thickness of similar to 100 mu m and light reflectance as low as 0.36% and independent of the incidence angle. The formation of such structures is rationalized based on delignification method, lignin content, carbonization temperature and wood density. Moreover, our measurements indicate a laser beam reflectivity lower than commercial light stoppers in current use. Overall, the wood-based superblack material is introduced as a mechanically robust surrogate for microfabricated carbon nanotube arrays.
引用
收藏
页数:12
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