Additive effects of CuPcX4-TCNQ on CH3NH3PbI3 perovskite solar cells

被引：1

作者：

Suzuki, Atsushi ^{[1
]}

Hasegawa, Ryota ^{[1
]}

Funayama, Kai ^{[1
]}

Oku, Takeo ^{[1
]}

Okita, Masanobu ^{[2
]}

Fukunishi, Sakiko ^{[2
]}

Tachikawa, Tomoharu ^{[2
]}

Hasegawa, Tomoya ^{[2
]}

机构：

[1] Univ Shiga Prefecture, 2500 Hassaka, Hikone, Shiga 5228533, Japan

[2] Osaka Gas Chem Co Ltd, 5-11-61 Torishima,Konohana Ku, Osaka 5540051, Japan

来源：

JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS | 2023年 / 34卷 / 07期

关键词：

EFFICIENCY; PHTHALOCYANINE; LEAD; PERFORMANCE; STABILITY; PORPHYRIN; IMPACT;

D O I：

10.1007/s10854-023-10001-z

中图分类号：

TM [电工技术]; TN [电子技术、通信技术];

学科分类号：

0808 ; 0809 ;

摘要：

Fabrication and characterization of methylammonium lead iodide CH3NH3PbI3 (MAPbI(3)) perovskite solar cells using decaphenylpentacyclosilane (DPPS), metal phthalocyanine complex doped with tetracyanoquinodimethane (TCNQ) as hole-transporting materials were performed. Additive effects of carboxylic acid, amino, or sulfonic acid sodium salt substituted phthalocyanine complex (MPcX4, M = Cu, Zn, Co, X = COOH, NH2 or SO3Na) doped with TCNQ on the photovoltaic properties, crystal orientation, morphologies and electronic structure were investigated. Incorporation of DPPS and CuPc(NH2)(4) doped with TCNQ on the perovskite layer promoted the carrier generation and charge transfer, yielding the best performance of conversion efficiency as compared with other cases. The photovoltaic performance depended on the (100) crystal orientation in the perovskite layer. The surface modification and passivation in the perovskite layer supported the photovoltaic performance with stability under air atmosphere. The molecular interaction based on overlap of pi-orbital on CuPc(NH2)(4), TCNQ and the perovskite crystal promoted the charge transfer at the interface between the perovskite layer and hole-transporting layer, improving the photovoltaic performance.

引用

页数：20

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