A practical perspective on the potential of rechargeable Mg batteries

被引:57
作者
Blazquez, J. Alberto [1 ]
Maca, Rudi R. [1 ]
Leonet, Olatz [1 ]
Azaceta, Eneko [1 ]
Mukherjee, Ayan [2 ]
Zhao-Karger, Zhirong [3 ,4 ]
Li, Zhenyou [3 ,4 ]
Kovalevsky, Aleksey [5 ]
Fernandez-Barquin, Ana [1 ]
Mainar, Aroa R. [1 ]
Jankowski, Piotr [6 ]
Rademacher, Laurin [7 ]
Dey, Sunita [8 ]
Dutton, Sian E. [9 ]
Grey, Clare P. [8 ]
Drews, Janina [7 ]
Haecker, Joachim [7 ]
Danner, Timo [3 ,7 ]
Latz, Arnulf [3 ,7 ,10 ]
Sotta, Dane [11 ]
Palacin, M. Rosa [12 ]
Martin, Jean-Frederic
Lastra, Juan Maria Garcia [6 ,11 ]
Fichtner, Maximilian [3 ,4 ]
Kundu, Sumana [13 ,14 ]
Kraytsberg, Alexander [13 ,14 ]
Ein-Eli, Yair [13 ,14 ]
Noked, Malachi [2 ]
Aurbach, Doron [2 ]
机构
[1] CIDETEC, Basque Res & Technol Alliance BRTA, Parque Cientif & Tecnol Gipuzkoa, Paseo Miramon, 196, San Sebastian 20014, Spain
[2] Bar Ilan Univ, Dept Chem, IL-5290002 Ramat Gan, Israel
[3] Helmholtz Inst Ulm HIU Electrochem Energy Storage, D-89081 Ulm, Germany
[4] Karlsruhe Inst Technol KIT, Inst Nanotechnol INT, D-76021 Karlsruhe, Germany
[5] Technion R&D Fdn LTD, Israel Inst Met, Technion City, IL-3200003 H_efa, Israel
[6] Tech Univ Denmark, Dept Energy Convers & Storage, Lyngby, Denmark
[7] German Aerosp Ctr DLR, Inst Engn Thermodynam, Pfaffenwaldring 38-40, D-70569 Stuttgart, Germany
[8] Univ Cambridge, Dept Chem, Cambridge CB2, England
[9] Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge, Cambridgeshire, England
[10] Ulm Univ, Inst Electrochem, D-89081 Ulm, Germany
[11] CEA LITEN, 17 Rue Martyrs, F-38054 Grenoble 9, France
[12] ICMAB CSIC, Inst Ciencia Mat Barcelona, Campus UAB, Catalonia 08193, Spain
[13] Technion Israel Inst Technol, Dept Mat Sci & Engn, JJ Thomson Ave, IL-3200003 H_aifa, Israel
[14] Technion Israel Inst Technol, Grand Technion Energy Program GTEP, IL-3200003 H_efa, Israel
关键词
HIGH ANODIC STABILITY; MAGNESIUM ALLOYS; LI-ION; ELECTROLYTE-SOLUTIONS; REVERSIBLE MAGNESIUM; CORROSION BEHAVIOR; CATHODE MATERIALS; SULFUR BATTERIES; INTERCALATION; EFFICIENT;
D O I
10.1039/d2ee04121a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Emerging energy storage systems based on abundant and cost-effective materials are key to overcome the global energy and climate crisis of the 21st century. Rechargeable Magnesium Batteries (RMB), based on Earth-abundant magnesium, can provide a cheap and environmentally responsible alternative to the benchmark Li-ion technology, especially for large energy storage applications. Currently, RMB technology is the subject of intense research efforts at laboratory scale. However, these emerging approaches must be placed in a real-world perspective to ensure that they satisfy key technological requirements. In an attempt to bridge the gap between laboratory advancements and industrial development demands, herein, we report the first non-aqueous multilayer RMB pouch cell prototypes and propose a roadmap for a new advanced RMB chemistry. Through this work, we aim to show the great unrealized potential of RMBs.
引用
收藏
页码:1964 / 1981
页数:18
相关论文
共 140 条
[91]  
Moseley PT, 2015, ELECTROCHEMICAL ENERGY STORAGE FOR RENEWABLE SOURCES AND GRID BALANCING, P1
[92]   Corrosion of magnesium electrolytes: chlorides - the culprit [J].
Muldoon, John ;
Bucur, Claudiu B. ;
Oliver, Allen G. ;
Zajicek, Jaroslav ;
Allred, Gary D. ;
Boggess, William C. .
ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (02) :482-487
[93]   First investigation of indium-based electrode in Mg battery [J].
Murgia, Fabrizio ;
Weldekidan, Ephrem Terefe ;
Stievano, Lorenzo ;
Monconduit, Laure ;
Berthelot, Romain .
ELECTROCHEMISTRY COMMUNICATIONS, 2015, 60 :56-59
[94]   Alloy Anode Materials for Rechargeable Mg Ion Batteries [J].
Niu Jiazheng ;
Zhang Zhonghua ;
Aurbach, Doron .
ADVANCED ENERGY MATERIALS, 2020, 10 (23)
[95]   Polyanthraquinone-Based Organic Cathode for High-Performance Rechargeable Magnesium-Ion Batteries [J].
Pan, Baofei ;
Huang, Jinhua ;
Feng, Zhenxing ;
Zeng, Li ;
He, Meinan ;
Zhang, Lu ;
Vaughey, John T. ;
Bedzyk, Michael J. ;
Fenter, Paul ;
Zhang, Zhengcheng ;
Burrell, Anthony K. ;
Liao, Chen .
ADVANCED ENERGY MATERIALS, 2016, 6 (14)
[96]   Hydrides for solid-state batteries: A review [J].
Pang, Y. ;
Liu, Y. ;
Yang, J. ;
Zheng, S. ;
Wang, C. .
MATERIALS TODAY NANO, 2022, 18
[97]  
PANG Y, 2022, SCI CHINA MATER
[98]   Investigation on the formation of Mg metal anode/electrolyte interfaces in Mg/S batteries with electrolyte additives [J].
Parambath, Vinayan Bhaghavathi ;
Zhao-Karger, Zhirong ;
Diemant, Thomas ;
Jaeckle, Markus ;
Li, Zhenyou ;
Scherer, Torsten ;
Gross, Axel ;
Behm, R. Juergen ;
Fichtner, Maximilian .
JOURNAL OF MATERIALS CHEMISTRY A, 2020, 8 (43) :22998-23010
[99]   Influence of microstructure and composition on the corrosion behaviour of Mg/Al alloys in chloride media [J].
Pardo, A. ;
Merino, M. C. ;
Coy, A. E. ;
Viejo, F. ;
Arrabal, R. ;
Feliu, S., Jr. .
ELECTROCHIMICA ACTA, 2008, 53 (27) :7890-7902
[100]   Review-Polymer Electrolytes for Magnesium Batteries: Forging Away from Analogs of Lithium Polymer Electrolytes and Towards the Rechargeable Magnesium Metal Polymer Battery [J].
Park, Bumjun ;
Schaefer, Jennifer L. .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2020, 167 (07)