A practical perspective on the potential of rechargeable Mg batteries

被引：57

作者：

Blazquez, J. Alberto ^{[1
]}

Maca, Rudi R. ^{[1
]}

Leonet, Olatz ^{[1
]}

Azaceta, Eneko ^{[1
]}

Mukherjee, Ayan ^{[2
]}

Zhao-Karger, Zhirong ^{[3
,4
]}

Li, Zhenyou ^{[3
,4
]}

Kovalevsky, Aleksey ^{[5
]}

Fernandez-Barquin, Ana ^{[1
]}

Mainar, Aroa R. ^{[1
]}

Jankowski, Piotr ^{[6
]}

Rademacher, Laurin ^{[7
]}

Dey, Sunita ^{[8
]}

Dutton, Sian E. ^{[9
]}

Grey, Clare P. ^{[8
]}

Drews, Janina ^{[7
]}

Haecker, Joachim ^{[7
]}

Danner, Timo ^{[3
,7
]}

Latz, Arnulf ^{[3
,7
,10
]}

Sotta, Dane ^{[11
]}

Palacin, M. Rosa ^{[12
]}

Martin, Jean-Frederic

Lastra, Juan Maria Garcia ^{[6
,11
]}

Fichtner, Maximilian ^{[3
,4
]}

Kundu, Sumana ^{[13
,14
]}

Kraytsberg, Alexander ^{[13
,14
]}

Ein-Eli, Yair ^{[13
,14
]}

Noked, Malachi ^{[2
]}

Aurbach, Doron ^{[2
]}

机构：

[1] CIDETEC, Basque Res & Technol Alliance BRTA, Parque Cientif & Tecnol Gipuzkoa, Paseo Miramon, 196, San Sebastian 20014, Spain

[2] Bar Ilan Univ, Dept Chem, IL-5290002 Ramat Gan, Israel

[3] Helmholtz Inst Ulm HIU Electrochem Energy Storage, D-89081 Ulm, Germany

[4] Karlsruhe Inst Technol KIT, Inst Nanotechnol INT, D-76021 Karlsruhe, Germany

[5] Technion R&D Fdn LTD, Israel Inst Met, Technion City, IL-3200003 H_efa, Israel

[6] Tech Univ Denmark, Dept Energy Convers & Storage, Lyngby, Denmark

[7] German Aerosp Ctr DLR, Inst Engn Thermodynam, Pfaffenwaldring 38-40, D-70569 Stuttgart, Germany

[8] Univ Cambridge, Dept Chem, Cambridge CB2, England

[9] Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge, Cambridgeshire, England

[10] Ulm Univ, Inst Electrochem, D-89081 Ulm, Germany

[11] CEA LITEN, 17 Rue Martyrs, F-38054 Grenoble 9, France

[12] ICMAB CSIC, Inst Ciencia Mat Barcelona, Campus UAB, Catalonia 08193, Spain

[13] Technion Israel Inst Technol, Dept Mat Sci & Engn, JJ Thomson Ave, IL-3200003 H_aifa, Israel

[14] Technion Israel Inst Technol, Grand Technion Energy Program GTEP, IL-3200003 H_efa, Israel

来源：

ENERGY & ENVIRONMENTAL SCIENCE | 2023年 / 16卷 / 05期

关键词：

HIGH ANODIC STABILITY; MAGNESIUM ALLOYS; LI-ION; ELECTROLYTE-SOLUTIONS; REVERSIBLE MAGNESIUM; CORROSION BEHAVIOR; CATHODE MATERIALS; SULFUR BATTERIES; INTERCALATION; EFFICIENT;

D O I：

10.1039/d2ee04121a

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Emerging energy storage systems based on abundant and cost-effective materials are key to overcome the global energy and climate crisis of the 21st century. Rechargeable Magnesium Batteries (RMB), based on Earth-abundant magnesium, can provide a cheap and environmentally responsible alternative to the benchmark Li-ion technology, especially for large energy storage applications. Currently, RMB technology is the subject of intense research efforts at laboratory scale. However, these emerging approaches must be placed in a real-world perspective to ensure that they satisfy key technological requirements. In an attempt to bridge the gap between laboratory advancements and industrial development demands, herein, we report the first non-aqueous multilayer RMB pouch cell prototypes and propose a roadmap for a new advanced RMB chemistry. Through this work, we aim to show the great unrealized potential of RMBs.

引用

页码：1964 / 1981

页数：18

共 140 条

[1] Ahmad AH, 2009, AIP CONF PROC, V1136, P31, DOI 10.1063/1.3160156
[2] Electrodeposited Bi, Sb and Bi1-xSbx alloys as anodes for Mg-ion batteries
Arthur, Timothy S.
Singh, Nikhilendra
Matsui, Masaki
[J]. ELECTROCHEMISTRY COMMUNICATIONS, 2012, 16 (01) : 103 - 106
[3] Determination of Average Coulombic Efficiency for Rechargeable Metal Anodes in Prospective Solutions
Attias, Ran
Dlugatch, Ben
Blumen, Omer
Shwartsman, Keren
Salama, Michal
Shpigel, Netanel
Sharon, Daniel
[J]. ACS APPLIED MATERIALS & INTERFACES, 2022, 14 (27) : 30952 - 30961
[4] The Role of Surface Adsorbed Cl- Complexes in Rechargeable Magnesium Batteries
Attias, Ran
Chae, Munseok S.
Dlugatch, Ben
Oliel, Matan
Goffer, Yosef
Aurbach, Doron
[J]. ACS CATALYSIS, 2020, 10 (14): : 7773 - 7784
[5] Modulation, Characterization, and Engineering of Advanced Materials for Electrochemical Energy Storage Applications: MoO3/V2O5 Bilayer Model System
Attias, Ran
Salama, Michael
Pant, Reeta
Gofer, Yossef
Aurbach, Doron
[J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2019, 123 (27) : 16577 - 16587
[6] Anode-Electrolyte Interfaces in Secondary Magnesium Batteries
Attias, Ran
Salama, Michael
Hirsch, Baruch
Goffer, Yosef
Aurbach, Doron
[J]. JOULE, 2019, 3 (01) : 27 - 52
[7] Prototype systems for rechargeable magnesium batteries
Aurbach, D
Lu, Z
Schechter, A
Gofer, Y
Gizbar, H
Turgeman, R
Cohen, Y
Moshkovich, M
Levi, E
[J]. NATURE, 2000, 407 (6805) : 724 - 727
[8] GAPLESS PEIERLS TRANSITION
BATRA, IP
[J]. PHYSICAL REVIEW B, 1990, 42 (14) : 9162 - 9165
[9] Bell N., 2017, MAGNESIUM RECYCLING, P1
[10] Theoretical versus Practical Energy: A Plea for More Transparency in the Energy Calculation of Different Rechargeable Battery Systems
Betz, Johannes
Bieker, Georg
Meister, Paul
Placke, Tobias
Winter, Martin
Schmuch, Richard
[J]. ADVANCED ENERGY MATERIALS, 2019, 9 (06)

← 1 2 3 4 5 6 7 8 9 10 →