Constructing a highly tough, durable, and renewable flexible filter by epitaxial growth of a glass fiber fabric for high flux and superefficient oil-water separation

被引:12
作者
Wang, Yiwen [1 ]
Meng, Fanxiang [1 ]
Han, Lei [1 ]
Liu, Xiangyu [1 ]
Guo, Fang [1 ]
Lu, Hang [1 ]
Cheng, Dehao [1 ]
Wang, Wenbo [1 ]
机构
[1] Inner Mongolia Univ, Coll Chem & Chem Engn, Hohhot 010021, Peoples R China
基金
中国国家自然科学基金;
关键词
Underwater superoleophobic; Glass-fiber fabric; Oil-water separation; Epitaxial growth; Silicate; OIL/WATER SEPARATION; COATED MESHES; DESIGN; SILICATE; SURFACE; OXIDE;
D O I
10.1016/j.jhazmat.2023.130807
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The separation and purification of complex and stable stubborn oily sewage is extremely challenging. To respond to this challenge, we developed a powerful flexible filter with ultrahigh strength, durability, flux, separation efficiency, and a multiobjective separation function based on a universal epitaxial growth process of glass fiber fabric (Gf). The underwater oil contact angle (UOCA) of the silicate@Gf (MgSi@Gf) filter is 156.3(?), so it can achieve both an ultrahigh permeation flux (5632.7 L.m(- 2).h(-1)) and oil-water separation efficiency (99.5%) under gravity (asymptotic to 1 kPa) in purifying surfactant-stabilized emulsions, actual industrial oily sewage and mechanical cold rolling emulsions. The filter with a high tensile strength (66.5 MPa) and oil invasion pressure (4626 Pa) can withstand the impact of much sewage or intense water flow. The filter can tolerate extreme conditions and can maintain high separation performance in acid or alkaline (pH 1-13), high or low temperature (100 C-?, 200 C-?,-18 C-?) conditions or natural salty waters such as seawater. The filter can remove methylene blue (MB) dye (99.8%) by filtration, and can be repeatedly and easily reconstructed (renewable advantage). The filter shows great potential for efficiently eliminating the hazards of contaminants in actual oily sewage and thus protect human health.
引用
收藏
页数:13
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共 78 条
[1]   Improved water resource management framework for water sustainability and security [J].
Ahmed, Sameh S. ;
Bali, Rekha ;
Khan, Hasim ;
Mohamed, Hassan Ibrahim ;
Sharma, Sunil Kumar .
ENVIRONMENTAL RESEARCH, 2021, 201
[2]   Multifunctional membranes with super-wetting characteristics for oil-water separation and removal of hazardous environmental pollutants from water: A review [J].
Baig, Umair ;
Faizan, Muhammad ;
Sajid, Mohd .
ADVANCES IN COLLOID AND INTERFACE SCIENCE, 2020, 285
[3]   Kinetics of dissolution of glass fibre in hot alkaline solution [J].
Bashir, S. T. ;
Yang, L. ;
Liggat, J. J. ;
Thomason, J. L. .
JOURNAL OF MATERIALS SCIENCE, 2018, 53 (03) :1710-1722
[4]   Characterization of magnesium silicate hydrate (M-S-H) [J].
Bernard, Ellina ;
Lothenbach, Barbara ;
Chlique, Christophe ;
Wyrzykowski, Mateusz ;
Dauzeres, Alexandre ;
Pochard, Isabelle ;
Cau-Dit-Coumes, Celine .
CEMENT AND CONCRETE RESEARCH, 2019, 116 :309-330
[5]   Application of Phase-Selective Organogelators (PSOGs) for Marine Oil Spill Remediation [J].
Bi, Huifang ;
An, Chunjiang ;
Mulligan, Catherine N. ;
Chen, Zhi ;
Lee, Kenneth ;
Wen, Jiyuan ;
Qu, Zhaonian ;
Chen, Xinya .
JOURNAL OF MARINE SCIENCE AND ENGINEERING, 2022, 10 (08)
[6]   Oil-in-water emulsion breaking marine bacteria for demulsifying oily wastewater [J].
Cai, Qinhong ;
Zhu, Zhiwen ;
Chen, Bing ;
Zhang, Baiyu .
WATER RESEARCH, 2019, 149 :292-301
[7]   Facile design of a stable and inorganic underwater superoleophobic copper mesh modified by self-assembly sodium silicate and aluminum oxide for oil/water separation with high flux [J].
Cao, Huaijie ;
Liu, Ying .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2021, 598 :483-491
[8]   Energy performance factors in wastewater treatment plants: A review [J].
Cardoso, Bruno J. ;
Rodrigues, Eugenio ;
Gaspar, Adelio R. ;
Gomes, Alvaro .
JOURNAL OF CLEANER PRODUCTION, 2021, 322 (322)
[9]   Separation Mechanism and Construction of Surfaces with Special Wettability for Oil/Water Separation [J].
Chen, Chaolang ;
Weng, Ding ;
Mahmood, Awais ;
Chen, Shuai ;
Wang, Jiadao .
ACS APPLIED MATERIALS & INTERFACES, 2019, 11 (11) :11006-11027
[10]   Nacre-Inspired Mineralized Films with High Transparency and Mechanically Robust Underwater Superoleophobicity [J].
Chen, Wei ;
Zhang, Pengchao ;
Zang, Ruhua ;
Fan, Junbing ;
Wang, Shutao ;
Wang, Bailiang ;
Meng, Jingxin .
ADVANCED MATERIALS, 2020, 32 (11)