Activity Regulation of Fenton/Fenton-like Reactions in Single-Atom Catalysis

被引：10
作者：
Liang, Xiao [1 ]
Wang, Dingsheng [1 ]
机构：
[1] Tsinghua Univ, Engn Res Ctr Adv Rare Earth Mat, Dept Chem, Beijing 100084, Peoples R China
来源：
CHEMCATCHEM | 2023年 / 15卷 / 11期
基金：
中国国家自然科学基金; 国家重点研发计划;
关键词：
Fenton-like reactions; single-atom catalysts; organics degradation; tumor therapy; OXYGEN REDUCTION; DOPED CARBON; SITES; ELECTROCATALYSTS; COORDINATION; EFFICIENT; GRAPHENE; DESIGN;
D O I：
10.1002/cctc.202201579
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
On the one hand, Fenton-like reactions are common side reactions in electrocatalytic oxygen reduction reaction (ORR). The generated reactive oxygen species (ROS) could damage the active sites of single-atom catalysts (SACs), thereby affecting the stability of the catalysts. On the other hand, the Fenton-like reaction could generate radicals with strong oxidative properties, which could be used in the degradation of pollutants and tumor therapy. In this review, we summarize strategies to limit the occurrence of Fenton-like reactions and improve the stability of SACs. In addition, the promotion of Fenton-like reactivity of SACs and its application in related fields are also concluded.
引用
收藏
页数：18
相关论文
共 145 条
  • [1] Pyrrolic N-Stabilized Monovalent Ni Single-Atom Electrocatalyst for Efficient CO2 Reduction: Identifying the Role of Pyrrolic-N and Synergistic Electrocatalysis
    Boppella, Ramireddy
    Austeria, Muthu P.
    Kim, Yujin
    Kim, Eunhyo
    Song, Inae
    Eom, Yaeeun
    Kumar, D. Praveen
    Balamurugan, Mani
    Sim, Eunji
    Kim, Do Hwan
    Kim, Tae Kyu
    [J]. ADVANCED FUNCTIONAL MATERIALS, 2022, 32 (35)
  • [2] Recent advances of cancer chemodynamic therapy based on Fenton/Fenton-like chemistry
    Cao, Changyu
    Wang, Xiaorui
    Yang, Nan
    Song, Xuejiao
    Dong, Xiaochen
    [J]. CHEMICAL SCIENCE, 2022, 13 (04) : 863 - 889
  • [3] High-Efficiency Electrocatalysis of Molecular Oxygen toward Hydroxyl Radicals Enabled by an Atomically Dispersed Iron Catalyst
    Cao, Peike
    Quan, Xie
    Zhao, Kun
    Chen, Shuo
    Yu, Hongtao
    Su, Yan
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2020, 54 (19) : 12662 - 12672
  • [4] The cathode catalysts of hydrogen fuel cell: From laboratory toward practical application
    Cao, Shuang
    Sun, Tong
    Li, Jin-Rong
    Li, Qin-Zhu
    Hou, Chun-Chao
    Sun, Qi
    [J]. NANO RESEARCH, 2023, 16 (04) : 4365 - 4380
  • [5] Nitrogen-coordinated single-atom catalysts with manganese and cobalt sites for acidic oxygen reduction
    Chao, Guojie
    Zhang, Yizhe
    Zhang, Longsheng
    Zong, Wei
    Zhang, Nan
    Xue, Tiantian
    Fan, Wei
    Liu, Tianxi
    Xie, Yi
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2022, 10 (11) : 5930 - 5936
  • [6] Regulating electronic structure of CoN4 with axial Co-S for promoting oxygen reduction and Zn-air battery performance
    Chen, Chang
    Chen, Zhiqiang
    Zhong, Junxi
    Song, Xin
    Chen, Dongfang
    Liu, Shoujie
    Cheong, Weng-Chon
    Li, Jiazhan
    Tan, Xin
    He, Chang
    Zhang, Jiaqi
    Liu, Di
    Yuan, Qiuhua
    Chen, Chen
    Peng, Qing
    Li, Yadong
    [J]. NANO RESEARCH, 2023, 16 (04) : 4211 - 4218
  • [7] Single-Atom Iron Anchored Tubular g-C3N4 Catalysts for Ultrafast Fenton-Like Reaction: Roles of High-Valency Iron-Oxo Species and Organic Radicals
    Chen, Fei
    Liu, Lian-Lian
    Wu, Jing-Hang
    Rui, Xian-Hong
    Chen, Jie-Jie
    Yu, Yan
    [J]. ADVANCED MATERIALS, 2022, 34 (31)
  • [8] Molecular Engineering toward Pyrrolic N-Rich M-N4 (M = Cr, Mn, Fe, Co, Cu) Single-Atom Sites for Enhanced Heterogeneous Fenton-Like Reaction
    Chen, Feng
    Wu, Xi-Lin
    Shi, Chenyang
    Lin, Hongjun
    Chen, Jianrong
    Shi, Yanpeng
    Wang, Shaobin
    Duan, Xiaoguang
    [J]. ADVANCED FUNCTIONAL MATERIALS, 2021, 31 (13)
  • [9] MOF Encapsulating N-Heterocyclic Carbene-Ligated Copper Single-Atom Site Catalyst towards Efficient Methane Electrosynthesis
    Chen, Shenghua
    Li, Wen-Hao
    Jiang, Wenjun
    Yang, Jiarui
    Zhu, Jiexin
    Wang, Liqiang
    Ou, Honghui
    Zhuang, Zechao
    Chen, Mingzhao
    Sun, Xiaohui
    Wang, Dingsheng
    Li, Yadong
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2022, 61 (04)
  • [10] Atomic-Level Modulation of Electronic Density at Cobalt Single-Atom Sites Derived from Metal-Organic Frameworks: Enhanced Oxygen Reduction Performance
    Chen, Yuanjun
    Gao, Rui
    Ji, Shufang
    Li, Haijing
    Tang, Kun
    Jiang, Peng
    Hu, Haibo
    Zhang, Zedong
    Hao, Haigang
    Qu, Qingyun
    Liang, Xiao
    Chen, Wenxing
    Dong, Juncai
    Wang, Dingsheng
    Li, Yadong
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2021, 60 (06) : 3212 - 3221
12345678910