Ceramizable phenolic adhesive modified by different inorganic particles: A comparative study of thermal stability, bonding strength and bonding mechanism

被引：18

作者：

Wang, Cunku ^{[1
]}

Ding, Jie ^{[1
,2
]}

Huang, Zhixiong ^{[1
]}

Zhuang, Yingluo ^{[1
]}

Li, Yan ^{[1
]}

Shi, Minxian ^{[1
]}

Qin, Yan ^{[1
]}

机构：

[1] Wuhan Univ Technol, Sch Mat Sci & Engn, Wuhan 430070, Peoples R China

[2] Luoshi Rd 122, Wuhan, Hubei, Peoples R China

来源：

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY | 2023年 / 43卷 / 01期

关键词：

Phenolic adhesive; Inorganic particles; Bonding strength; Ceramization; Bonding mechanism; RESISTANT ORGANIC ADHESIVE; TEMPERATURE; CERAMICS; PERFORMANCE; POLYMER; RESIN; COMPOSITES; PYROLYSIS; TOUGHNESS; REPAIR;

D O I：

10.1016/j.jeurceramsoc.2022.09.034

中图分类号：

TQ174 [陶瓷工业]; TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

In this work, two ceramizable phenolic adhesives were prepared using ZrSi2 particles or ZrSi2/B4C mix particles as the inorganic fillers. The thermal stability, bonding strength, microstructure and phase composition of the adhesives were investigated by TGA, shear strength of Al2O3 joints, SEM, EDS, XRD and XPS. The results show that these two adhesives have different bonding performances and ceramicization evolutions above 600 degrees C in air due to the addition of the second phase particles B4C. The bonding strength of ZrSi2/B4C modified phenolic adhesive after treatment at 1200 celcius can be as high as 36.6 MPa, while the bonding strength of ZrSi2 modified phenolic adhesive under the same conditions is only 17.5 MPa. B4C undergoes oxidation reaction before ZrSi2, and the oxidation product B2O3 liquid phase not only reacts with ZrSi2 to form oxidation-resistant ZrB2, but also can dissolve the high temperatures defects of the adhesive and chemically bond with the Al2O3 substrates at the interface.

引用

页码：64 / 72

页数：9

共 32 条

[1] SiAlON ceramics from preceramic polymers and nano-sized fillers: Application in ceramic joining [J].

Bernardo, E. ;

Parcianello, G. ;

Colombo, R. ;

Adair, J. H. ;

Barnes, A. T. ;

Hellmann, J. R. ;

Jones, B. H. ;

Kruise, J. ;

Swab, J. J. .

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY, 2012, 32 (07) :1329-1335

[2] The effects of zirconium diboride particles on the ablation performance of carbon-phenolic composites under an oxyacetylene flame [J].

Chen, Yaxi ;

Hong, Changqing ;

Chen, Ping .

RSC ADVANCES, 2013, 3 (33) :13734-13739

[3] ZrB2-SiC-G Composite Prepared by Spark Plasma Sintering of In-Situ Synthesized ZrB2-SiC-C Composite Powders [J].

Cheng, YeHong ;

Qi, Yushi ;

Hu, Ping ;

Zhou, Shanbao ;

Chen, Guiqing ;

An, Jiadong ;

Jin, Kunfeng ;

Han, Wenbo .

JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 2016, 99 (06) :2131-2137

[4] Surface generation in high-speed grinding of brittle and tough ceramics [J].

Choudhary, Amit ;

Paul, Soumitra .

CERAMICS INTERNATIONAL, 2021, 47 (21) :30546-30562

[5] Structure-charring relationship in phenol-formaldehyde type resins [J].

Costa, L ;

diMontelera, LR ;

Camino, G ;

Weil, ED ;

Pearce, EM .

POLYMER DEGRADATION AND STABILITY, 1997, 56 (01) :23-35

[6] Influence of B4C on oxidation resistance of PSN/borosilicate glass-B4C field-based repair coating of C/C aircraft brake materials at 700-900 °C [J].

Deng, Juanli ;

Hu, Kaiyue ;

Lu, Baofu ;

Zheng, Bohan ;

Fan, Shangwu ;

Zhang, Litong ;

Cheng, Laifei .

CERAMICS INTERNATIONAL, 2019, 45 (16) :20860-20872

[7] A novel glass-ceramic with high crystallinity for joining of SiC ceramic [J].

Fang, Jian ;

Zhang, Jie ;

Liu, Chunfeng ;

Sun, Liangbo .

MATERIALS LETTERS, 2020, 277

[8] Joining of engineering ceramics [J].

Fernie, J. A. ;

Drew, R. A. L. ;

Knowles, K. M. .

INTERNATIONAL MATERIALS REVIEWS, 2009, 54 (05) :283-331

[9] X-ray photoelectron spectroscopy investigation of boron carbide films deposited by sputtering [J].

Jacobsohn, LG ;

Schulze, RK ;

da Costa, MEHM ;

Nastasi, M .

SURFACE SCIENCE, 2004, 572 (2-3) :418-424

[10] Improved Adhesive Strength and Toughness of Polyvinyl Acetate Glue on Addition of Small Quantities of Graphene [J].

Khan, Umar ;

May, Peter ;

Porwal, Harshit ;

Nawaz, Khalid ;

Coleman, Jonathan N. .

ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (04) :1423-1428

← 1 2 3 4 →