Enhancement TiO2 photocatalytic hydrogen production via using ABO3 to construct heterojunction

被引:7
作者
Peng, Ke [1 ]
Yu, Shuohan [1 ]
Luo, Yongping [2 ]
Zhang, Aiqin [1 ]
Xie, Yu [1 ]
Luo, Yunxia [1 ]
Ling, Yun [1 ]
Zhao, Jinsheng [3 ]
机构
[1] Nanchang Hangkong Univ, Coll Environm & Chem Engn, Nanchang 330063, Peoples R China
[2] Huzhou Coll, Sch Intelligent Mfg, Huzhou 313000, Peoples R China
[3] Liaocheng Univ, Shandong Key Lab Chem Energy Storage & Novel Cell, Liaocheng 252059, Peoples R China
基金
中国国家自然科学基金;
关键词
TiO2; nanotubes; ABO(3); Type II heterojunction; Photocatalytic hydrogen production; SRTIO3; HETEROSTRUCTURES; NANOFIBERS; PERFORMANCE; WATER;
D O I
10.1016/j.colsurfa.2023.132822
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The lower photogenerated carrier separation efficiency seriously hinders the photocatalytic performance of TiO2. In order to solve this problem, we utilized SrTiO3 particles with low cost, good response to visible light, tunable band structure, and type II heterojunction with TiO2 to improve the photogenerated carrier separation efficiency of TiO2 in this study. The TiO2/SrTiO3 heterojunctions have a larger specific surface area than pristine TiO2, pristine SrTiO3. The results confirmed that the formation of heterostructures reduce the interfacial resistance of charge transfer; the transient and effectively improve the electron-hole pair separation efficiency. The hydrogen production efficiency of TiO2/SrTiO3 heterojunction composite is 807.7 mu molg(-1)h(-1), which is 26 times higher than pure TiO2 nanotubes. This work provides a new way to prepare efficient and low-cost photocatalysts using ABO(3).
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收藏
页数:9
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