energy dissipation;
gas content;
gas vortex;
mass transfer coefficient;
mass transfer;
numerical simulation;
paddle stirrer;
phase interface;
stirring power;
MASS-TRANSFER COEFFICIENT;
HYDRODYNAMIC CHARACTERISTICS;
VORTEX BEHAVIOR;
HOLD-UP;
FLOW;
PARAMETERS;
VESSELS;
REACTOR;
STAGE;
AREA;
D O I:
10.3390/chemengineering7020030
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
This article presents the results of hydrodynamics and mass exchange in a stirred tank upon the introduction of gas from an open gas vortex cavity into local liquid regions with reduced pressure. It establishes conditions for the intensive dispersion of gas. Velocity fields and liquid pressure behind the stirrer paddles are determined by numerical simulation in OpenFOAM. The gas content value, gas bubble diameters, and phase surface are determined experimentally. The stirrer power criterion is calculated by taking into account the gas content and power input. The experimental mass transfer data based on the absorption of atmospheric oxygen into water during the dispersion of gas from the open vortex cavity in the local liquid regions behind the rotating stirrer paddles are presented. In this case, the energy dissipation from the rotating stirrer reaches 25 W/kg, with a phase surface of 1000 m(-1) and a surface mass transfer coefficient of up to 0.3 center dot 10(-3) m/s. These parameters are obviously higher than the data obtained in the apparatus for mass exchange through surface vorticity. The advantage of the given method for gas dispersion in a liquid is the functional stability of the apparatus regardless of how deep the stirrer is immersed in the liquid or the temperature or pressure of the gas. Apparatuses based on the intensive gas dispersion method allow for varying the mass transfer coefficient and gas content across a broad range of values. This allows establishing a dependency between the experimentally obtained mass transfer coefficient, energy dissipation, and phase surface values. An equation for calculating the mass transfer coefficient is formulated by taking into account the geometric parameters of the stirrer apparatus based on the stirring power and phase surface values.
机构:
Curtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, AustraliaCurtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, Australia
Prakash, Baranivignesh
Bhatelia, Tejas
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Curtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, AustraliaCurtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, Australia
Bhatelia, Tejas
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Wadnerkar, Divyamaan
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Shah, Milinkumar T.
Pareek, Vishnu K.
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Curtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, AustraliaCurtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, Australia
Pareek, Vishnu K.
Utikar, Ranjeet P.
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Curtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, AustraliaCurtin Univ, Western Australia Sch Mines Minerals Energy & Che, Perth, WA 6845, Australia
机构:
Iowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USAIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Hu, Xiaofei
Ilgun, Aziz Dogan
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Iowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Iowa State Univ, Dept Chem & Biol Engn, 618 Bissell Rd, Ames, IA 50011 USAIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Ilgun, Aziz Dogan
Passalacqua, Alberto
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Iowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USAIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Passalacqua, Alberto
Fox, Rodney O.
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Iowa State Univ, Dept Chem & Biol Engn, 618 Bissell Rd, Ames, IA 50011 USAIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Fox, Rodney O.
Bertola, Francesco
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SABIC, Urmonderbaan 22,POB 319, NL-6160 AH Geleen, NetherlandsIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Bertola, Francesco
Milosevic, Miran
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SABIC, Urmonderbaan 22,POB 319, NL-6160 AH Geleen, NetherlandsIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
Milosevic, Miran
Visscher, Frans
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SABIC, Urmonderbaan 22,POB 319, NL-6160 AH Geleen, NetherlandsIowa State Univ, Dept Mech Engn, 2529 Union Dr, Ames, IA 50011 USA
机构:
Zhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Henan Acad Geol, Zhengzhou 450016, Peoples R China
Henan Inst Ultrapure Mineral Mat, Zhengzhou 450016, Peoples R China
Henan Ultrapure Mineral New Mat Ind Res Inst Co Lt, Sanmenxia 472000, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Huang, Yehao
Gao, Mingwei
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机构:
Wuhan Univ Sci & Technol, Hubei Key Lab Efficient Utilizat & Agglomerat Meta, Wuhan 430081, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Gao, Mingwei
Shang, Baozhong
论文数: 0引用数: 0
h-index: 0
机构:
Henan Acad Geol, Zhengzhou 450016, Peoples R China
Henan Inst Ultrapure Mineral Mat, Zhengzhou 450016, Peoples R China
Henan Ultrapure Mineral New Mat Ind Res Inst Co Lt, Sanmenxia 472000, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Shang, Baozhong
Yao, Jia
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Zhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Yao, Jia
Peng, Weijun
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Zhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Peng, Weijun
Song, Xiangyu
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Zhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China
Song, Xiangyu
Mei, Dan
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机构:
Wuhan Univ Sci & Technol, Hubei Key Lab Efficient Utilizat & Agglomerat Meta, Wuhan 430081, Peoples R ChinaZhengzhou Univ, Sch Chem Enginerring, Zhengzhou 450001, Peoples R China