Anode electrode;
Gas diffusion;
Gas distribution;
Gradient channel;
SOFC;
DUSTY-GAS;
PERFORMANCE;
PREDICTION;
FICKS;
D O I:
10.1016/j.ces.2023.119558
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
Precise geometrical adjustment of an anode is crucial for optimizing the performance of solid oxide fuel cell (SOFC). Fuel gas components of SOFC, including H-2, CH4, CO, CO2 and H2O, are complex in composition but play a significant role in determining the efficiency of SOFC. This study examines the fuel transport and distribution and the resultant SOFC performance by constructing various gradient channel anode (GCA) structures. The findings show that compared to the traditional un-gradient channel anode (un-GCA) cell, the GCA cell results in more uniform gas distribution and better diffusion of fuel gases, particularly H-2, CH4 and H2O. Because of the improved gas diffusion in the anode electrode, the GCA (12 mu m) cell exhibits a 2.34 % improvement in power density compared to the un-GCA cell at 800 degrees C and 0.6 V. Additionally, after increasing the mole fractions of H-2 and CH4 in the fuel gas, the power density of the GCA (12 mu m) cell is improved by 2.42 % compared with that of the un-GCA cell under the same condition. This study provides clear evidence that incorporating the gradient channel structure in the anode can effectively enhance gas transport, minimize localized gas aggregation and eventually improve the performance of SOFC.
机构:
Univ Tokyo, Inst Ind Sci, Meguro Ku, Tokyo 1538505, JapanUniv Tokyo, Grad Sch Engn, Dept Mech Engn, Bunkyo Ku, Tokyo 1138656, Japan
Shikazono, Naoki
Nakao, Masayuki
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机构:
Univ Tokyo, Grad Sch Engn, Dept Mech Engn, Bunkyo Ku, Tokyo 1138656, JapanUniv Tokyo, Grad Sch Engn, Dept Mech Engn, Bunkyo Ku, Tokyo 1138656, Japan
机构:
Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Res Inst Ind Sci & Technol RIST, Fuel Cell Project, Pohang 790600, Gyeongbuk, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Lim, H. -T.
Hwang, S. C.
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机构:
Res Inst Ind Sci & Technol RIST, Fuel Cell Project, Pohang 790600, Gyeongbuk, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Hwang, S. C.
Jung, M. G.
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机构:
Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Jung, M. G.
Park, H. W.
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机构:
Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Park, H. W.
Park, M. Y.
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机构:
Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Park, M. Y.
Lee, S. -S.
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Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea
Lee, S. -S.
Jung, Y. -G.
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h-index: 0
机构:
Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South KoreaChangwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea