Spatial and species-specific responses of biogenic volatile organic compound (BVOC) emissions to elevated ozone from 2014-2020 in China

被引:14
作者
Li, Lingyu [1 ]
Cao, Jing [1 ]
Hao, Yufang [2 ]
机构
[1] Qingdao Univ, Coll Environm Sci & Engn, Carbon Neutral & Ecoenvironm Technol Innovat Ctr Q, Qingdao 266071, Peoples R China
[2] Paul Scherrer Inst ETH, Energy & Environm Res Div, Lab Atmospher Chem, CH-5232 Villigen, Switzerland
基金
中国国家自然科学基金;
关键词
Biogenic emission; VOCs; Stressed emission; MEGAN3; 1; Ozone exposure; SPATIOTEMPORAL VARIATION; ATMOSPHERIC CHEMISTRY; TROPOSPHERIC OZONE; ISOPRENE EMISSION; AMBIENT OZONE; MEGAN MODEL; EXPOSURE; POLLUTION; SUMMERTIME; AEROSOLS;
D O I
10.1016/j.scitotenv.2023.161636
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
China suffered from serious and elevated ozone (O3) pollution during 2014-2020. O3 exposure increased with W126, a biologically based cumulative exposure index, at a rate of 1.738 ppm-hr yr-1. MEGAN3.1 was applied to estimate bio-genic volatile organic compound (BVOC) emissions and their response to O3 pollution in China by quantifying species responses to O3 stress. In 2020, China's BVOC emissions were 23.26 Tg when considering the effects of O3 pollution, which was 1.7 % higher than that without O3 stress. Isoprene, monoterpenes, sesquiterpenes, and other VOC emissions changed by -1.0 %, 1.4 %, 15.5 %, and 2.7 %, respectively. The stimulated BVOC emissions were mainly focused on the North China Plain (NCP) and a partial area of the Tibetan Plateau, which increased by >45 %. Changes in monthly emissions differed, with the greatest increase, 181 tons (3.25 %), in August. The seasonal patterns for the impacts of O3 pollution were also distinguished spatially. The elevated O3 exposure caused BVOC emission increases of 104.7 Gg yr-1 during 2014-2020, with isoprene, monoterpenes, sesquiterpenes, and other VOCs contributing -18.6 %, 27.5 %, 40.4 %, and 50.8 %, respectively. The greatest increase in emissions appeared on the NCP and eastern and central China, with annual increases of >100 tons per grid (36 km x 36 km). The interannual variations in BVOC emissions also displayed different seasonal patterns.
引用
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页数:9
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