Carrier Cooling in Lead Halide Perovskites: A Perspective on Hot Carrier Solar Cells

被引：23

作者：

Lin, Weihua ^{[1
,2
]}

Canton, Sophie E. ^{[3
]}

Zheng, Kaibo ^{[1
,2
,3
]}

Pullerits, Tonu ^{[1
,2
]}

机构：

[1] Lund Univ, Chem Phys, S-22100 Lund, Sweden

[2] Lund Univ, NanoLund, S-22100 Lund, Sweden

[3] Tech Univ Denmark, Dept Chem, DK-2800 Lyngby, Denmark

来源：

ACS ENERGY LETTERS | 2023年 / 9卷 / 01期

基金：

瑞典研究理事会;

关键词：

DETAILED BALANCE LIMIT; QUANTUM-WELLS; EFFICIENCY; RELAXATION; CONVERSION; ELECTRONS; TRANSPORT; EXCITONS; POLARONS; TANDEM;

D O I：

10.1021/acsenergylett.3c02359

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The concept of hot carrier solar cells (HCSCs) has been proposed as a promising yet elusive path toward high-performance photovoltaics (PV), capable of surpassing the Shockley-Queisser limit by recycling energy that would otherwise be lost during thermalization. Lead halide perovskites (LHPs) have emerged as highly promising materials for PV applications. The reports of slow hot carrier (HC) cooling in these materials have ignited discussions of their potential in realizing HCSCs. Here we summarize the key findings regarding HC dynamics in LHPs, as revealed by numerous studies using advanced time-resolved spectroscopies. We also emphasize the interconnected mechanisms involved in HC cooling. In addition, we discuss the influence of nanostructuring on HC cooling dynamics in LHPs and suggest that two-dimensional LHPs, with their inherent quantum well structure, might exhibit modified phononic features and altered carrier-phonon coupling strength. We conclude by critically discussing the prospects for HCSCs, taking into account our current understanding of HC cooling and excitation conditions under sunlight.

引用

页码：298 / 307

页数：10

共 101 条

[1] The effect of Auger heating on intraband carrier relaxation in semiconductor quantum rods [J].

Achermann, Marc ;

Bartko, Andrew P. ;

Hollingsworth, Jennifer A. ;

Klimov, Victor I. .

NATURE PHYSICS, 2006, 2 (08) :557-561

[2] NTMpy: An open source package for solving coupled parabolic differential equations in the framework of the three-temperature model [J].

Alber, Lukas ;

Scalera, Valentino ;

Unikandanunni, Vivek ;

Schick, Daniel ;

Bonetti, Stefano .

COMPUTER PHYSICS COMMUNICATIONS, 2021, 265

[3] Third Generation Photovoltaics based on Multiple Exciton Generation in Quantum Confined Semiconductors [J].

Beard, Matthew C. ;

Luther, Joseph M. ;

Semonin, Octavi E. ;

Nozik, Arthur J. .

ACCOUNTS OF CHEMICAL RESEARCH, 2013, 46 (06) :1252-1260

[4] Scaling law for excitons in 2D perovskite quantum wells [J].

Blancon, J. -C. ;

Stier, A. V. ;

Tsai, H. ;

Nie, W. ;

Stoumpos, C. C. ;

Traore, B. ;

Pedesseau, L. ;

Kepenekian, M. ;

Katsutani, F. ;

Noe, G. T. ;

Kono, J. ;

Tretiak, S. ;

Crooker, S. A. ;

Katan, C. ;

Kanatzidis, M. G. ;

Crochet, J. J. ;

Even, J. ;

Mohite, A. D. .

NATURE COMMUNICATIONS, 2018, 9

[5] PEROVSKITE PHYSICS Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites [J].

Blancon, J. -C. ;

Tsai, H. ;

Nie, W. ;

Stoumpos, C. C. ;

Pedesseau, L. ;

Katan, C. ;

Kepenekian, M. ;

Soe, C. M. M. ;

Appavoo, K. ;

Sfeir, M. Y. ;

Tretiak, S. ;

Ajayan, P. M. ;

Kanatzidis, M. G. ;

Even, J. ;

Crochet, J. J. ;

Mohite, A. D. .

SCIENCE, 2017, 355 (6331) :1288-1291

[6] Quantifying Photoinduced Polaronic Distortions in Inorganic Lead Halide Perovskite Nanocrystals [J].

Cannelli, Oliviero ;

Colonna, Nicola ;

Puppin, Michele ;

Rossi, Thomas C. ;

Kinschel, Dominik ;

Leroy, Ludmila M. D. ;

Loeffler, Janina ;

Budarz, James M. ;

March, Anne Marie ;

Doumy, Gilles ;

Al Haddad, Andre ;

Tu, Ming-Feng ;

Kumagai, Yoshiaki ;

Walko, Donald ;

Smolentsev, Grigory ;

Krieg, Franziska ;

Boehme, Simon C. ;

Kovalenko, Maksym, V ;

Chergui, Majed ;

Mancini, Giulia F. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2021, 143 (24) :9048-9059

[7] Uncovering the Electron-Phonon Interplay and Dynamical Energy-Dissipation Mechanisms of Hot Carriers in Hybrid Lead Halide Perovskites [J].

Chan, Christopher C. S. ;

Fan, Kezhou ;

Wang, Han ;

Huang, Zhanfeng ;

Novko, Dino ;

Yan, Keyou ;

Xu, Jianbin ;

Choy, Wallace C. H. ;

Loncaric, Ivor ;

Wong, Kam Sing .

ADVANCED ENERGY MATERIALS, 2021, 11 (09)

[8] Strong band filling induced significant excited state absorption in MAPbI3 under high pump power [J].

Chen, B. A. ;

Pang, G. T. ;

Lan, X. Q. ;

He, Z. B. ;

Chen, R. .

MATERIALS TODAY PHYSICS, 2020, 14

[9] Two-photon absorption in halide perovskites and their applications [J].

Chen, Junsheng ;

Zhang, Wei ;

Pullerits, Tonu .

MATERIALS HORIZONS, 2022, 9 (09) :2255-2287

[10] Cation-Dependent Hot Carrier Cooling in Halide Perovskite Nanocrystals [J].

Chen, Junsheng ;

Messing, Maria E. ;

Zheng, Kaibo ;

Pullerits, Tonu .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2019, 141 (08) :3532-3540

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