Preparation and catalytic properties of ZnO/Na0.5Bi0.5TiO3 composites

被引:6
作者
Wang, Baolong [1 ,2 ]
Hong, Ying [1 ,2 ]
Hu, Shanshan [1 ,2 ]
Lu, Shuang [1 ,2 ]
Gu, Chenzhang [1 ,2 ]
Wu, Qi [1 ,2 ]
Chu, Benli [1 ,2 ]
Wang, Yinzhen [1 ,2 ]
机构
[1] South China Normal Univ, Guangdong Engn Technol Res Ctr Efficient Green Ene, Sch Phys & Telecommun Engn, Guangdong Prov Key Lab Quantum Engn & Quantum Mat, Guangzhou 510006, Peoples R China
[2] South China Normal Univ, Guangdong Hong Kong Joint Lab Quantum Matter, Guangzhou 510006, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
Na0; 5Bi0; 5TiO3; ZnO; MB degradation; Z-scheme heterojunction; Photocatalysis; RAY PHOTOELECTRON-SPECTROSCOPY; PHOTOCATALYTIC DEGRADATION; ZNO NANOSTRUCTURES; DESIGN; NA0.5BI0.5TIO3; NANOSHEETS; NANORODS; ENERGY; WATER;
D O I
10.1016/j.vacuum.2022.111632
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
ZnO/Na0.5Bi0.5TiO3 composites were prepared by chemical hydrothermal deposition and hydrothermal method and the effects of ZnO adding on the properties of Na0.5Bi0.5TiO3 were investigated. The results show that the ZnO/Na0.5Bi0.5TiO3 composite with 5% ZnO content has the best photocatalytic performance and good cycling stability. Under simulated sunlight irradiation, the degradation rate for MB (10 mg/L) by ZnO/Na0.5Bi0.5TiO3 composites reached 100% within 20 minutes, and the reaction rate constant was 0.07427min- 1, which were 27.51 and 6.00 times higher than those of Na0.5Bi0.5TiO3 (NBT, 0.0027 min-1) and ZnO (0.01237min- 1), respectively. The incorporation of ZnO on the Na0.5Bi0.5TiO3 can form Z-scheme heterostructure ZnO/ Na0.5Bi0.5TiO3 and increase the specific surface area, inhibiting the recombination of electron and hole and improving separation and transfer carriers efficiency. ZnO/Na0.5Bi0.5TiO3 composites have potential applications in high-efficiency and high-activity photocatalysts to degrade organic pollutants.
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页数:10
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共 43 条
  • [1] Tunable emission of LiCa3MgV3O12:Bi3+ via energy transfer and changing excitation wavelength
    Cao, Renping
    Chen, Tao
    Ren, Yongchun
    Liao, Chenxing
    Luo, Zhiyang
    Ye, Yuanxiu
    Guo, Yimin
    [J]. MATERIALS RESEARCH BULLETIN, 2019, 111 : 87 - 92
  • [2] Self-assembly synthesis of CuO/ZnO hollow microspheres and their photocatalytic performance under natural sunlight
    Chen, Chuansheng
    Liu, Xiaoyan
    Fang, Qun
    Chen, Xiaohua
    Liu, Tiangui
    Zhang, Mansi
    [J]. VACUUM, 2020, 174
  • [3] One-pot synthesis of Bi2TiO4F2/BiOBr ferroelectric heterostructure for photocatalytic oxygen evolution
    Chen, Jifang
    Liu, Huan
    Zhu, Liuyang
    Fu, Zhengping
    Lu, Yalin
    [J]. JOURNAL OF ALLOYS AND COMPOUNDS, 2021, 873
  • [4] Synthesis flower-like BiVO4/BiOI core/shell heterostructure photocatalyst for tetracycline degradation under visible-light irradiation
    Chen, Yongyang
    Liu, Yonggang
    Xie, Xin
    Li, Chen
    Si, Yushan
    Zhang, Menghan
    Yan, Qishe
    [J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2019, 30 (10) : 9311 - 9321
  • [5] Degradation of methylene blue and methyl orange by palladium-doped TiO2 photocatalysis for water reuse: Efficiency and degradation pathways
    Chi Hieu Nguyen
    Fu, Chun-Chieh
    Juang, Ruey-Shin
    [J]. JOURNAL OF CLEANER PRODUCTION, 2018, 202 : 413 - 427
  • [6] The novel n-n type BiOCl0.8I0.2/Bi5O7I heterojunction composite photocatalysts with high photocatalytic capacity for pollutants
    Cui, Baolong
    Sun, Xinyue
    Li, Shu
    Xue, Lu
    Hu, Yingyue
    Du, Yi
    [J]. VACUUM, 2022, 204
  • [7] SnO2 doped ZnO nanostructures for highly efficient photocatalyst
    Faisal, M.
    Ibrahim, Ahmed A.
    Harraz, Farid A.
    Bouzid, Houcine
    Al-Assiri, M. S.
    Ismail, Adel A.
    [J]. JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2015, 397 : 19 - 25
  • [8] The same chemical state of carbon gives rise to two peaks in X-ray photoelectron spectroscopy
    Greczynski, G.
    Hultman, L.
    [J]. SCIENTIFIC REPORTS, 2021, 11 (01)
  • [9] Reliable determination of chemical state in x-ray photoelectron spectroscopy based on sample-work-function referencing to adventitious carbon: Resolving the myth of apparent constant binding energy of the C 1s peak
    Greczynski, G.
    Hultman, L.
    [J]. APPLIED SURFACE SCIENCE, 2018, 451 : 99 - 103
  • [10] C1s Peak of Adventitious Carbon Aligns to the Vacuum Level: Dire Consequences for Material's Bonding Assignment by Photoelectron Spectroscopy
    Greczynski, Grzegorz
    Hultman, Lars
    [J]. CHEMPHYSCHEM, 2017, 18 (12) : 1507 - 1512