Novel polyamide-hydrazide based reverse osmosis membrane with enhanced antifouling properties

被引:12
作者
Wang, Zhongyang [1 ,2 ]
Akram, Muhammad Adnan [1 ]
Zhang, Shanshan [1 ]
Gong, Jingwei [3 ]
Zhao, Lihua [1 ]
Liu, Zhiyu [1 ,4 ]
Niu, Q. Jason [1 ]
机构
[1] Shenzhen Univ, Inst Adv Study, Shenzhen 518060, Peoples R China
[2] Shenzhen Univ, Coll Civil & Transportat Engn, Shenzhen 518061, Peoples R China
[3] Univ Malaya, Fac Engn, Dept Chem Engn, 50603 Kuala Lumpur, Malaysia
[4] Shenzhen Univ, Coll Chem & Environm Engn, Shenzhen 518060, Peoples R China
基金
中国国家自然科学基金;
关键词
Reverse osmosis membrane; Antifouling; Novel monomer; Polyamide-hydrazide; Morphology control; FILM COMPOSITE MEMBRANES; SEPARATION PERFORMANCE; SURFACE; MORPHOLOGY; TRANSPORT; LAYER;
D O I
10.1016/j.desal.2023.117233
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The typical "ridge-valley" structure of traditional reverse osmosis (RO) membranes ensures good permeability with high risk of inducing membrane fouling. It is a challenge to develop a smooth RO membrane without loss of permeability. In this study, cyclobutane-1,2,3,4-tetracarbohydrazide (CBTH) was designed and synthesized, and a composite RO membrane based on CBTH and cyclobutane-1,2,3,4-tetracarboxylic acid chloride (BTC) was constructed. The CBTH-BTC membrane exhibits a smooth selective layer with thickness of 45 nm. The desalination performance test results show that the CBTH-BTC membrane has permeability and desalination performance comparable to the traditional RO membrane (the water permeability coefficient reaches 3.0 L & sdot;m(- 2)& sdot;h(- 1)& sdot;bar(-1), and the rejection of NaCl reaches 99.2 %). Importantly, the hydrophilic and smooth surface imparts the membrane with good antifouling properties to hydrophilic, hydrophobic and surfactant pollutants. In this study, RO membranes with good permeability and excellent antifouling performance were successfully prepared from the perspective of reaction monomer design, which provides a new idea to regulate the morphology and antifouling properties of RO membranes.
引用
收藏
页数:11
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