Perspective on powder technology for all-solid-state batteries: How to pair sulfide electrolyte with high-voltage cathode

被引：33
作者：
Hu, Jiangkui [1 ,2 ]
Yang, Shijie [1 ,2 ]
Pei, Yingying [1 ,2 ]
Wang, Xilong [1 ,2 ]
Liao, Yulong [1 ,2 ]
Li, Shuai [1 ,2 ]
Yue, Aolong [1 ,2 ]
Huang, Jia-Qi [1 ,2 ]
Yuan, Hong [1 ,2 ]
机构：
[1] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China
[2] Beijing Inst Technol, Adv Res Inst Multidisciplinary Sci, Beijing 100081, Peoples R China
来源：
PARTICUOLOGY | 2024年 / 86卷
基金：
中国国家自然科学基金; 北京市自然科学基金;
关键词：
Sulfide solid electrolytes; High-voltage cathodes; Electrode/electrolyte interfaces; All-solid-state lithium batteries; LITHIUM ION BATTERIES; POLYMER ELECTROLYTES; THERMAL RUNAWAY; INTERFACE STABILITY; PERFORMANCE; CONDUCTOR; CHEMISTRY; CAPACITY; LAYER; INTERPHASE;
D O I：
10.1016/j.partic.2023.04.005
中图分类号：
TQ [化学工业];
学科分类号：
0817 ;
摘要：
Sulfide solid electrolytes (SEs) have attracted ever-increasing attention due to their superior roomtemperature ionic conductivity (similar to 10-2 S cm(-1)). Additionally, the integration of sulfide SEs and highvoltage cathodes is promising to achieve higher energy density. However, the incompatible interfaces between sulfide SEs and high-voltage cathodes have been one of the key factors limiting their applications. Therefore, this review presents a critical summarization of the interfacial issues in all-solid-state lithium batteries based on sulfide SEs and high-voltage cathodes and proposes strategies to stabilize the electrolyte/cathode interfaces. Moreover, the future research direction of electrolyte/cathode interfaces and application prospects of powder technology in sulfide-based ASSLBs were also discussed.
引用
收藏
页码：55 / 66
页数：12
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