Influence of the Distance between two Catalysts for CO2 to Dimethyl Ether Tandem Reaction

被引：2
|
作者：
Javed, Mudassar [1 ]
Broesigke, Georg [1 ]
Schomaecker, Reinhard [2 ]
Repke, Jens-Uwe [1 ]
机构：
[1] Tech Univ Berlin, Proc Dynam & Operat Grp, Str 17 Juni 135, D-10623 Berlin, Germany
[2] Tech Univ Berlin, Inst Chem, Str 17 Juni 135, D-10623 Berlin, Germany
来源：
CHEMICAL ENGINEERING & TECHNOLOGY | 2023年 / 46卷 / 06期
关键词：
Dimethyl ether tandem system; HZSM-5; deactivation; Mass transfer; Methanol; Tandem catalysis; CARBON-DIOXIDE; METHANOL; DEHYDRATION; CONVERSION; ACID; DME; SYNGAS; ENERGY; HYDROGENATION; ZEOLITES;
D O I：
10.1002/ceat.202200541
中图分类号：
TQ [化学工业];
学科分类号：
0817 ;
摘要：
Tandem reactions, with their great potential for reduction of capital and operational costs, reaction time, and byproducts are becoming more prominent. Among possible tandem reaction systems for direct conversion of CO2 to green fuel, dimethyl ether synthesis via methanol route is of vital importance. However, there are several parameters which must be considered for the combination of two catalysts to achieve promising performance, of those, the distance between the two catalysts is a crucial one. This distance can affect the overall performance of the tandem system by causing external mass transfer limitations or the poisoning of the catalysts. This work presents a systematic study on the influence of the distance between the two catalysts for the CO2 to dimethyl ether tandem system.
引用
收藏
页码：1163 / 1169
页数：7
相关论文
共 50 条
  • [21] CO2 to dimethyl ether (DME): structural and functional insights of hybrid catalysts
    Ghosh, Anindya
    Nag, Debjani
    Chatterjee, Rupak
    Singha, Aniruddha
    Dash, Pratik Swarup
    Choudhury, Biswajit
    Bhaumik, Asim
    CATALYSIS SCIENCE & TECHNOLOGY, 2024, 14 (06) : 1387 - 1427
  • [22] Hydrogenation of CO2 to Dimethyl Ether over Bronsted Acidic PdZn Catalysts
    Bahruji, Hasliza
    Armstrong, Robert D.
    Esquius, Jonathan Ruiz
    Jones, Wilm
    Bowker, Michael
    Hutchings, Graham J.
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2018, 57 (20) : 6821 - 6829
  • [23] Hybrid monometallic and bimetallic copper-palladium zeolite catalysts for direct synthesis of dimethyl ether from CO2
    Navarro-Jaen, Sara
    Virginie, Mirella
    Morin, Jean-Charles
    Thuriot-Roukos, Joelle
    Wojcieszak, Robert
    Khodakov, Andrei Y.
    NEW JOURNAL OF CHEMISTRY, 2022, 46 (08) : 3889 - 3900
  • [24] Direct synthesis of dimethyl ether from CO2 hydrogenation over novel hybrid catalysts containing a Cu-ZnO-ZrO2 catalyst admixed with WOx/Al2O3 catalysts: Effects of pore size of Al2O3 support and W loading content
    Suwannapichat, Yossapon
    Numpilai, Thanapa
    Chanlek, Narong
    Faungnawakij, Kajornsak
    Chareonpanich, Metta
    Limtrakul, Jumras
    Witoon, Thongthai
    ENERGY CONVERSION AND MANAGEMENT, 2018, 159 : 20 - 29
  • [25] Direct CO2-to-dimethyl Ether Hydrogenation over CuZnZr/zeolite Hybrid Catalyst: New Evidences on the Interaction Between Acid and Metal Sites
    Catizzone, Enrico
    Bonura, Giuseppe
    Migliori, Massimo
    Braccio, Giacobbe
    Frusteri, Francesco
    Giordano, Girolamo
    ANNALES DE CHIMIE-SCIENCE DES MATERIAUX, 2019, 43 (03): : 141 - 149
  • [26] Selective hydrogenation of CO2 into dimethyl ether over hydrophobic and gallium-modified copper catalysts
    Li, Hangjie
    Xiao, Yuehua
    Xiao, Jiale
    Fan, Kai
    Li, Bingkuan
    Li, Xiaolong
    Wang, Liang
    Xiao, Feng-Shou
    CHINESE JOURNAL OF CATALYSIS, 2023, 54 : 178 - 187
  • [27] Dimethyl ether synthesis from CO2 hydrogenation over hybrid catalysts: effects of preparation methods
    Kornas, Agnieszka
    Grabowski, R.
    Sliwa, M.
    Samson, K.
    Ruggiero-Mikolajczyk, M.
    Zelazny, A.
    REACTION KINETICS MECHANISMS AND CATALYSIS, 2017, 121 (01) : 317 - 327
  • [28] Catalytic conversion of CO2 to dimethyl ether: A review of recent advances in catalysts and water selective layer
    Le, Ng Jia
    Fong, Yeong Yin
    JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2024, 140 : 88 - 102
  • [29] Direct Synthesis of Dimethyl Ether from CO2 Hydrogenation over Core-Shell Nanotube Bi-Functional Catalyst
    Mohamud, Mohamed Yusuf
    Abdullah, Tuan Amran Tuan
    Ahmad, Arshad
    Ikram, Muhammad
    Alir, Afizah
    Phey, Melissa Low Phey
    Nabgan, Walid
    CATALYSTS, 2023, 13 (02)
  • [30] Catalyst configuration for the direct synthesis of dimethyl ether from CO and CO2 hydrogenation on CuO-ZnO-MnO/SAPO-18 catalysts
    Ateka, Ainara
    Sanchez-Contador, Miguel
    Erena, Javier
    Aguayo, Andres T.
    Bilbao, Javier
    REACTION KINETICS MECHANISMS AND CATALYSIS, 2018, 124 (01) : 401 - 418
12345