A review of understanding electrocatalytic reactions in energy conversion and energy storage systems via scanning electrochemical microscopy

被引:9
作者
Park, Jihye [1 ]
Lim, Jong Hwan [1 ]
Kang, Jin-Hyuk [1 ]
Lim, Jiheon [1 ,2 ]
Jang, Ho Won [2 ]
Shin, Hosun [1 ,3 ]
Park, Sun Hwa [1 ,3 ]
机构
[1] Korea Res Inst Stand & Sci, Interdisciplinary Mat Measurement Inst, Daejeon 34113, South Korea
[2] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 08826, South Korea
[3] Univ Sci & Technol, Dept Appl Measurement Sci, Daejeon 34113, South Korea
来源
JOURNAL OF ENERGY CHEMISTRY | 2024年 / 91卷
关键词
Scanning electrochemical microscopy; Electrocatalyst; Electrocatalysis; Water splitting; Fuel cell; Metal-oxygen battery; HYDROGEN EVOLUTION REACTION; REDOX COMPETITION MODE; OXYGEN REDUCTION; SURFACE INTERROGATION; HYBRID NANOSTRUCTURES; CATALYTIC-ACTIVITY; CELL MICROSCOPY; COLLECTION MODE; DIFFUSION LAYER; ELECTROLYTE;
D O I
10.1016/j.jechem.2023.12.015
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
To address climate change and promote environmental sustainability, electrochemical energy conversion and storage systems emerge as promising alternative to fossil fuels, catering to the escalating demand for energy. Achieving optimal energy efficiency and cost competitiveness in these systems requires the strategic design of electrocatalysts, coupled with a thorough comprehension of the underlying mechanisms and degradation behavior occurring during the electrocatalysis processes. Scanning electrochemical microscopy (SECM), an analytical technique for studying surface electrochemically, stands out as a powerful tool offering electrochemical insights. It possesses remarkable spatiotemporal resolution, enabling the visualization of the localized electrochemical activity and surface topography. This review compiles crucial research findings and recent breakthroughs in electrocatalytic processes utilizing the SECM methodology, specifically focusing on applications in electrolysis, fuel cells, and metal-oxygen batteries within the realm of energy conversion and storage systems. Commencing with an overview of each energy system, the review introduces the fundamental principles of SECM, and aiming to provide new perspectives and broadening the scope of applied research by describing the major research categories within SECM. (c) 2023 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. This is an open access article under the CC BY -NC -ND license (http:// creativecommons.org/licenses/by-nc-nd/4.0/).
引用
收藏
页码:155 / 177
页数:23
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