Manganese-based oxide electrocatalysts for the oxygen evolution reaction: a review

被引：80

作者：

Wang, Peng ^{[1
,2
]}

Zhang, Shiqi ^{[1
,2
]}

Wang, Zhaobo ^{[1
,2
]}

Mo, Yuhan ^{[1
,2
]}

Luo, Xiaoyang ^{[1
,2
]}

Yang, Fan ^{[3
]}

Lv, Meili ^{[3
]}

Li, Zhaoxiang ^{[4
]}

Liu, Xuanwen ^{[1
]}

机构：

[1] Northeastern Univ, Sch Mat Sci & Engn, Shenyang 110819, Peoples R China

[2] Northeastern Univ Qinhuangdao, Sch Resources & Mat, Key Lab Dielect & Electrolyte Funct Mat Hebei Prov, Qinhuangdao 066004, Peoples R China

[3] Qinhuangdao Solid Waste Management Ctr, Qinhuangdao 066004, Peoples R China

[4] Qinhuangdao Capital Starlight Environm Technol Co, Qinhuangdao 066004, Peoples R China

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2023年 / 11卷 / 11期

基金：

中国国家自然科学基金;

关键词：

ELECTROCHEMICAL WATER OXIDATION; LAYERED DOUBLE HYDROXIDES; ZINC-ION BATTERY; BIFUNCTIONAL CATALYSTS; HIGHLY EFFICIENT; REDUCTION REACTION; RECENT PROGRESS; HIGH-CAPACITY; MN OXIDES; NI FOAM;

D O I：

10.1039/d2ta09039b

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The oxygen evolution reaction (OER), as an essential process in water decomposition and air batteries, has received increasing attention in the context of clean energy production and efficient energy storage. With their abundant composition and morphology, manganese-based oxides (MnOx) offer great possibilities for the exploration and design of OER catalysts. In this paper, three classes of MnOx materials, including MnO2, Mn2O3, and Mn3O4, are systematically reviewed and their development and applications in OER systems are comprehensively presented. Subsequently, the effects of Jahn-Teller distortion and the question of the active site and stability of MnOx in the OER are discussed, and the presence of Mn3+, which is considered essential for OER activity, and strategies for improving performance are proposed. This paper focuses on the impact of crystal structure, catalytic mechanisms, and design strategies on MnOx.

引用

页码：5476 / 5494

页数：19

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