Optical Properties of Fine Mode Aerosols over High-Altitude Himalayan Glacier Regions

被引:3
作者
Verma, Sushant Ranjan [1 ]
Pervez, Shamsh [1 ]
Chow, Judith C. [2 ,3 ]
Watson, John G. [2 ,3 ]
Andrabi, Syed Muzaffarali [4 ]
Mandal, Papiya [5 ]
Khan, Noor Afshan [5 ]
Tiwari, Suresh [6 ]
Chandra Dumka, Umesh [7 ]
Chakrabarty, Rajan K. [8 ]
Verma, Madhuri [1 ]
Pervez, Yasmeen Fatima [9 ]
Mishra, Archi [1 ]
Tamrakar, Aishwaryashri [1 ]
Sowmya, Hulivahana Nagaraju [10 ]
Deb, Manas Kanti [1 ]
Ghosh, Kallol K. [1 ]
Jain, Vikas Kumar [11 ]
Karbhal, Indrapal [1 ]
Shrivas, Kamlesh [1 ]
Satnami, Manmohan Lal [1 ]
机构
[1] Pt Ravishankar Shukla Univ, Sch Studies Chem, Raipur 492010, Chhattisgarh, India
[2] Desert Res Inst, Div Atmospher Sci, Reno, NV 89512 USA
[3] Chinese Acad Sci, Inst Earth & Environm, Xian 710061, Peoples R China
[4] Kashmir Univ, Srinagar 190006, Hazaratbal, India
[5] Natl Environm Engn Res Inst, Nagpur 440020, Maharashtra, India
[6] Indian Inst Trop Meteorol, Pune 411008, Maharashtra, India
[7] Aryabhatta Res Inst Observat Sci, Naini Tal 263001, Uttarakhand, India
[8] Washington Univ, Environm & Chem Engn, DOE, St Louis, MO 63130 USA
[9] Govt Dr Waman Wasudev Patankar Girls PG Coll, Durg 491001, Chhattisgarh, India
[10] Dayananda Sagar Coll Engn, Dept Civil Engn, Bangalore 560078, Karnataka, India
[11] Minist Skill Dev Tech Educ & Employment, Directorate Tech Educ, Atal Nagar Naya Raipur 492002, Chhattisgarh, India
来源
ACS EARTH AND SPACE CHEMISTRY | 2023年 / 7卷 / 08期
关键词
light-absorbing aerosols; carbonaceous matters; radiative forcing; Himalayan glacier; brownandblack carbon; BIOMASS BURNING EMISSIONS; LONG-RANGE TRANSPORT; LIGHT-ABSORPTION; BROWN CARBON; BLACK CARBON; ELEMENTAL CARBON; ORGANIC-CARBON; MANORA PEAK; VISIBILITY; PARTICLES;
D O I
10.1021/acsearthspacechem.3c00088
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Duringthe summer and winter periods of 2019-2020, we conductedsampling of fine mode ambient aerosols in the western Himalayan glacialregion (WHR; Thajiwas glacier, 2799 m asl), central Himalayan glacialregion (CHR; Gomukh glacier, 3415 m asl), and eastern Himalayan glacialregion (EHR; Zemu glacier, 2700 m asl). We evaluated the aerosol opticalproperties, which included the mass absorption coefficient, mass absorptionefficiency, mass scattering efficiency, absorption angstrom exponent,single scattering albedo, as well as their simple radiative forcingefficiencies. We observed the highest absorption in the near ultraviolet-visiblewavelength range (200-400 nm), with CHR showing the highestabsorption compared to the other two sites, WHR and EHR, respectively.Across the wavelength range of 200-1100 nm, the overall contributionof black carbon to light attenuation was greater than that of browncarbon. However, brown carbon dominated the absorption in the nearUV-visible wavelengths, providing evidence of its non-trivialpresence over the Himalayan region. Additionally, we observed a positiveradiative forcing (W/g), which leads to net warming at these sites.The findings of this ground-based study contribute to our understandingof the light-absorbing nature of carbonaceous aerosols and their impacton the Himalayan glacier regions.
引用
收藏
页码:1536 / 1544
页数:9
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