Preheated combustion characteristics and fuel-nitrogen conversion paths for bituminous coal and anthracite in wide-range preheating temperature

被引:20
作者
Zhang, Xiaoyu [1 ,2 ]
Zhu, Shujun [1 ]
Zhu, Jianguo [1 ,3 ]
Hui, Jicheng [1 ,4 ]
Liu, Yuhua [1 ,3 ]
Zhang, Jiahang [1 ,3 ]
Lin, Jiangong [1 ,5 ]
Lyu, Qinggang [1 ,3 ]
机构
[1] Chinese Acad Sci, Inst Engn Thermophys, Beijing 100190, Peoples R China
[2] Univ Sci & Technol China, Hefei 230026, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[4] North China Electic Power Univ, Beijing 102206, Peoples R China
[5] Shanxi Datong Univ, Datong 037009, Peoples R China
基金
中国国家自然科学基金;
关键词
Bituminous coal; Anthracite; Preheating temperature; Nitrogen conversion; Preheated combustion; PULVERIZED CHAR; NO EMISSIONS; MILD COMBUSTION; FLUIDIZED-BED; GASIFICATION; RELEASE; TAR;
D O I
10.1016/j.joei.2023.101222
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
In this study, the characteristics of preheated combustion and fuel-nitrogen (fuel-N) conversion paths in wide-range preheating temperature (700 degrees C-900 degrees C) for bituminous coal and anthracite were revealed during the preheated combustion. The conversion of fuel-N mainly underwent three procedures, including the conversion from fuel-N to char-nitrogen (char-N), tar-nitrogen (tar-N) and gas-nitrogen (gas-N) in the PCFB, the reduction from preheated fuel-N to N2 in the reduction region of combustor and the release of NOx from the char-N in the oxidation region of combustor. During the preheating, the highest conversion ratio from fuel-N to tar-N was 9.94% at the preheating temperature of 700 degrees C for bituminous coal. However, the conversion ratio from fuel-N to tar-N was below 2% for anthracite from 700 degrees C to 900 degrees C. Most of fuel-N was transformed into char-N and N2 during the preheating. Although higher preheating temperature promoted the conversion of fuel-N during the preheating, the reduction of char-N was inhibited due to the lower temperature of reduction region in the combustor for anthracite. The lowest concentration of NOx emission was 226.01 mg/m3(@ 6% O2) at the pre-heating temperature of 850 degrees C for anthracite.
引用
收藏
页数:11
相关论文
共 43 条
[1]   NO formation during co-combustion of coal with two thermally treated biomasses [J].
Allguren, Thomas ;
Andersson, Klas ;
Fry, Andrew ;
Eddings, Eric G. .
FUEL PROCESSING TECHNOLOGY, 2022, 235
[2]   Review on the progress in emission control technologies for the abatement of CO2, SOx and NOx from fuel combustion [J].
Asghar, Usama ;
Rafiq, Sikander ;
Anwar, Adeel ;
Iqbal, Tanveer ;
Ahmed, Ashfaq ;
Jamil, Farrukh ;
Khurram, M. Shahzad ;
Akbar, Majid Majeed ;
Farooq, Abid ;
Shah, Noor S. ;
Park, Young-Kwon .
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2021, 9 (05)
[3]  
Bai C., 2022, PLOS ONE, V237
[4]   Release of fuel-nitrogen during the gasification of Shenmu coal in O2 [J].
Chang, LP ;
Xie, KC ;
Li, CZ .
FUEL PROCESSING TECHNOLOGY, 2004, 85 (8-10) :1053-1063
[5]   COAL DEVOLATILIZATION DURING RAPID TRANSIENT HEATING .1. PRIMARY DEVOLATILIZATION [J].
CHEN, JC ;
NIKSA, S .
ENERGY & FUELS, 1992, 6 (03) :254-264
[6]   An experimental and theoretical study of NO heterogeneous reduction in the reduction zone of ammonia co-firing in a coal-fired boiler: Influence of CO [J].
Chen, Ping ;
Wang, Huichun ;
Jiang, Boyu ;
Wang, Ying ;
Gu, Mingyan ;
Chen, Guang ;
Huang, Xiangyong .
FUEL PROCESSING TECHNOLOGY, 2022, 231
[7]   Coupling coal pyrolysis with char gasification in a multi-stage fluidized bed to co-produce high-quality tar and syngas [J].
Chen, Zhaohui ;
Li, Yunjia ;
Lai, Dengguo ;
Geng, Sulong ;
Zhou, Qi ;
Gao, Shiqiu ;
Xu, Guangwen .
APPLIED ENERGY, 2018, 215 :348-355
[8]   The effects of particle size on flameless combustion characteristics and NOx emissions of semi-coke with coal [J].
Ding, Hongliang ;
Ouyang, Ziqu ;
Zhang, Xiaoyu ;
Zhu, Shujun .
FUEL, 2021, 297
[9]   Studies of the release rule of NOx precursors during gasification of coal and its char [J].
Feng, J ;
Li, WY ;
Xie, KC ;
Liu, MR ;
Li, CZ .
FUEL PROCESSING TECHNOLOGY, 2003, 84 (1-3) :243-254
[10]   Fuel nitrogen conversion in solid fuel fired systems [J].
Glarborg, P ;
Jensen, AD ;
Johnsson, JE .
PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 2003, 29 (02) :89-113