Engineering hosts for Zn anodes in aqueous Zn-ion batteries

被引：198
作者：
Zhu, Yunhai [1 ]
Liang, Guojin [2 ]
Cui, Xun [1 ]
Liu, Xueqin [1 ]
Zhong, Haixia [4 ]
Zhi, Chunyi [3 ]
Yang, Yingkui [1 ]
机构：
[1] Wuhan Text Univ, State Key Lab New Text Mat & Adv Proc Technol, Wuhan 430200, Peoples R China
[2] Chinese Acad Sci, Shenzhen Inst Adv Technol, Fac Mat Sci & Engn, Shenzhen 518055, Guangdong, Peoples R China
[3] City Univ Hong Kong, Dept Mat Sci & Engn, Kowloon, 83 Tat Chee Ave, Hong Kong, Peoples R China
[4] Chinese Acad Sci, State Key Lab Rare Earth Resource Utilizat, Changchun Inst Appl Chem, Changchun 130022, Peoples R China
来源：
ENERGY & ENVIRONMENTAL SCIENCE | 2024年 / 17卷 / 02期
基金：
中国国家自然科学基金;
关键词：
ZINC ANODE; HIGH-CAPACITY; ELECTROLYTE; CHALLENGES; STRATEGIES; CHEMISTRY; METALS; LIFE;
D O I：
10.1039/d3ee03584k
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Aqueous zinc-ion batteries (ZIBs) distinguish themselves among the numerous viable alternatives to lithium-ion batteries on account of their potential advantages, which encompass enhanced safety, cost-effectiveness, and eco-friendliness. However, the metal zinc (Zn) that makes ZIBs competitive is now being plagued by dendrite growth and spontaneous side reactions (hydrogen evolution reaction and water-induced corrosion). These unavoidable parasitic reactions degrade the output energy/power density and shorten the actual lifespan of the Zn anode, rendering it infeasible for ZIBs to access the practical energy storage system. Herein, we systematically summarize the host-design strategies for the Zn anode regarding substrate (accommodation of Zn deposits) and interface (protection of Zn anode) fabrications. In addition, for the purpose of developing a Zn anode that is chemically and electrochemically stable, we thoroughly elucidate the internal mechanisms of the regulation strategies while offering guidance for the rational design of Zn anodes. This review may suggest a prospective guideline for developing high-performance Zn anodes for use in sustainable ZIBs. This review systematically summarizes the host-design strategies for Zn anodes regarding substrate and interface fabrication, aiming to provide a prospective guideline for developing high-performance Zn anodes.
引用
收藏
页码：369 / 385
页数：18
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