Global impacts of aviation on air quality evaluated at high resolution

Aviation emissions cause global changes in air quality which have been estimated to result in similar to 58 000 premature mortalities per year, but this number varies by an order of magnitude between studies. The causes of this uncertainty include differences in the assessment of ozone exposure impacts and in how air quality changes are simulated, as well as the possibility that low-resolution ( similar to 400 km) global models may overestimate impacts compared to finer-resolution ( similar to 50 km) regional models. We use the GEOS-Chem High-Performance chemistry-transport model at a 50 km global resolution, an order of magnitude finer than recent assessments of the same scope, to quantify the air quality impacts of aviation with a single internally consistent global approach. We find that aviation emissions in 2015 resulted in 21 200 (95 % confidence interval due to health response uncertainty: 19 400-22 900) premature mortalities due to particulate matter exposure and 53 100 (36 000-69 900) due to ozone exposure. Compared to a prior estimate of 6800 ozone-related premature mortalities for 2006 our central estimate is increased by 5.6 times due to the use of updated epidemiological data, which includes the effects of ozone exposure during winter, and by 1.3 times due to increased aviation fuel burn. The use of fine (50 km) resolution increases the estimated impacts on both ozone and particulate-matter-related mortality by a further 20 % compared to coarse-resolution (400 km) global simulation, but an intermediate resolution (100 km) is sufficient to capture 98 % of impacts. This is in part due to the role of aviation-attributable ozone, which is long-lived enough to mix through the Northern Hemisphere and exposure to which causes 2.5 times as much health impact as aviation-attributable PM 2.5 . This work shows that the air quality impacts of civil aviation emissions are dominated by the hemisphere-scale response of tropospheric ozone to aviation NO x rather than local changes and that simulations at similar to 100 km resolution provide similar results to those at a 2 times finer spatial scale. However, the overall quantification of health impacts is sensitive to assumptions regarding the response of human health to exposure, and additional research is needed to reduce uncertainty in the physical response of the atmosphere to aviation emissions.