Amorphous Pt-decorated α-Fe2O3 sensor with superior triethylamine sensing performance prepared by a one-step impregnation method

被引:6
作者
Chen, Li [1 ]
Xie, Jie [1 ]
Wang, Zhuoyuan [1 ]
Zhao, Yingni [1 ]
Gou, Jiangmei [1 ]
Wu, Jiangtao [1 ]
机构
[1] Sichuan Normal Univ, Coll Chem & Mat Sci, Chengdu 610068, Peoples R China
基金
中国国家自然科学基金;
关键词
Amorphous Pt decorating; Triethylamine sensor; Impregnation method; CORE-SHELL NANORODS; ROOM-TEMPERATURE; FACILE SYNTHESIS; NANOPARTICLES; HETEROSTRUCTURE; ARCHITECTURES; ACETONE; FE2O3; AU;
D O I
10.1016/j.jallcom.2023.173330
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Noble metals are widely used additives to improve the sensing performance of conductometric metal oxide gas sensors. Although amorphous noble metal particles are expected to further improve the gas sensor response, common techniques often result in crystalline nanoparticles. Herein, an amorphous Pt nanoparticle-decorated alpha-Fe2O3 sensor was prepared via a temperature-controlled facile one-step impregnation method without the use of a reductant, surfactant, or subsequent thermal reduction. The amorphous Pt-functionalized alpha-Fe2O3 exhibited superior sensing performance to triethylamine, achieving 100 degrees C and 140 degrees C decreases in the optimal working temperature, and had better selectivity, with 22-fold and 14-fold improvements in gas response when compared to those of crystallized Pt-functionalized alpha-Fe2O3 and pristine alpha-Fe2O3, respectively. The as-prepared amorphous Pt-decorated alpha-Fe2O3 sensor showed great promise as a promising triethylamine sensor, and the newly developed facile impregnation method was shown to be an effective strategy to synthesize amorphous noble metal-decorated metal oxide gas sensors.
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页数:9
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