Composition-dependent catalytic behaviour of Pt-Pd alloy in transfer hydrogenation of carbonates at room-temperature

被引：0
作者：
Liu, Jiaxin [1 ]
Li, Chuang [1 ]
Niu, Hongyu [1 ]
Liang, Changhai [1 ]
机构：
[1] Dalian Univ Technol, Sch Chem Engn, Dalian 116024, Peoples R China
来源：
CATALYSIS SCIENCE & TECHNOLOGY | 2023年 / 13卷 / 02期
关键词：
REDUCTION; OXIDATION; PALLADIUM; GLUCOSE; SURFACE; ACID; CO2;
D O I：
10.1039/d2cy01825j
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Transfer hydrogenation of carbonates using glucose to produce formates and gluconates is an attractive pathway for valorising waste streams. The investigation reveals a cooperative catalytic mechanism and composition-dependent behaviour of PtxPdy/CNTs catalysts. Insights into the mechanism will allow transfer hydrogenation of carbonates at room temperature to be widely utilized.
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收藏
页码：310 / 314
页数：5
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共 33 条
  • [1] PtNi catalysts prepared via borohydride reduction for hydrogenation of benzene
    Abu Bakar, N. H. H.
    Bettahar, M. M.
    Abu Bakar, M.
    Monteverdi, S.
    Ismail, J.
    Alnot, M.
    [J]. JOURNAL OF CATALYSIS, 2009, 265 (01) : 63 - 71
  • [2] Efficient transfer hydrogenation of carbonate salts from glycerol using water-soluble iridium N-heterocyclic carbene catalysts
    Ainembabazi, Diana
    Wang, Kai
    Finn, Matthew
    Ridenour, James
    Voutchkova-Kostal, Adelina
    [J]. GREEN CHEMISTRY, 2020, 22 (18) : 6093 - 6104
  • [3] ELECTRONIC-STRUCTURE AND SURFACE KINETICS OF PALLADIUM HYDRIDE STUDIED WITH X-RAY PHOTOELECTRON-SPECTROSCOPY AND ELECTRON-ENERGY-LOSS SPECTROSCOPY
    BENNETT, PA
    FUGGLE, JC
    [J]. PHYSICAL REVIEW B, 1982, 26 (11): : 6030 - 6039
  • [4] Iridium complexes catalysed the selective dehydrogenation of glucose to gluconic acid in water
    Borja, Pilar
    Vicent, Cristian
    Baya, Miguel
    Garcia, Hermenegildo
    Mata, Jose A.
    [J]. GREEN CHEMISTRY, 2018, 20 (17) : 4094 - 4101
  • [5] Enhanced Oxygen Reduction and Methanol Oxidation Electrocatalysis over Bifunctional PtPdIr Mesoporous Hollow Nanospheres
    Deng, Kai
    Xu, You
    Dai, Zechuan
    Yu, Hongjie
    Yin, Shuli
    Wang, Ziqiang
    Li, Xiaonian
    Wang, Liang
    Wang, Hongjing
    [J]. CHEMISTRY-AN ASIAN JOURNAL, 2019, 14 (21) : 3868 - 3874
  • [6] Coupling Glucose Dehydrogenation with CO2 Hydrogenation by Hydrogen Transfer in Aqueous Media at Room Temperature
    Ding, Guodong
    Su, Ji
    Zhang, Cheng
    Tang, Kan
    Yang, Lisha
    Lin, Hongfei
    [J]. CHEMSUSCHEM, 2018, 11 (13) : 2029 - 2034
  • [7] Iridium Complex Catalyzed Hydrogen Production from Glucose and Various Monosaccharides
    Fujita, Ken-ichi
    Inoue, Takayoshi
    Tanaka, Toshiki
    Jeong, Jaeyoung
    Furukawa, Shohichi
    Yamaguchi, Ryohei
    [J]. CATALYSTS, 2021, 11 (08)
  • [8] Carbonates (bicarbonates)/reduced graphene oxide as anode materials for sodium-ion batteries
    Gu, Xin
    Yan, Chunliu
    Yan, Liting
    Cao, Lei
    Niu, Feier
    Liu, Dandan
    Dai, Pengcheng
    Li, Liangjun
    Yang, Jian
    Zhao, Xuebo
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2017, 5 (47) : 24645 - 24650
  • [9] Boosting Formate Production in Electrocatalytic CO2 Reduction over Wide Potential Window on Pd Surfaces
    Jiang, Bei
    Zhang, Xia-Guang
    Jiang, Kun
    Wu, De-Yin
    Cai, Wen-Bin
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2018, 140 (08) : 2880 - 2889
  • [10] Manganese Catalyzed Hydrogenation of Organic Carbonates to Methanol and Alcohols
    Kumar, Amit
    Janes, Trevor
    Espinosa-Jalapa, Noel Angel
    Milstein, David
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2018, 57 (37) : 12076 - 12080
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