What do we talk about, when we talk about single-crystal termination-dependent selectivity of Cu electrocatalysts for CO2 reduction? A data-driven retrospective

被引:2
作者
Rossi, Kevin [1 ]
机构
[1] Ecole Polytech Fed Lausanne, Inst Sci & Ingn Chim, CH-1950 Sion, Switzerland
关键词
ELECTROCHEMICAL REDUCTION; CARBON-DIOXIDE; CATALYSTS; ELECTROREDUCTION; DESIGN; HYDROCARBONS; PERFORMANCE; DISCOVERY; SURFACES;
D O I
10.1039/d2cp04576a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We mine from the literature experimental data on the CO2 electrochemical reduction selectivity of Cu single crystal surfaces. We then probe the accuracy of a machine learning model trained to predict faradaic efficiencies for 11 CO2 reduction reaction products, as a function of the applied voltage at which the reaction takes place, and the relative amounts of non equivalent surface sites, distinguished according to their nominal coordination. A satisfactory model accuracy is found only when discriminating data according to their provenance. On one hand, this result points at a qualitative agreement across reported experimental CO2 reduction reactions trends for single-crystal surfaces with well-defined terminations. On the other, this finding hints at the presence of differences in nominally identical catalysts and/or CO2 reduction reaction measurements, which result in quantitative disagreement between experiments.
引用
收藏
页码:6867 / 6876
页数:10
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