Ultra-High-Resolution Perovskite Quantum Dot Light-Emitting Diodes

被引:13
作者
Mao, Chaomin [1 ,2 ]
Ju, Songman [1 ,2 ]
Zheng, Jinping [1 ]
Zheng, Yueting [1 ]
Xu, Zhongwei [1 ]
Lin, Lihua [1 ,2 ]
Hu, Hailong [1 ,2 ]
Yang, Kaiyu [1 ,2 ]
Guo, Tailiang [1 ,2 ]
Li, Fushan [1 ,2 ]
机构
[1] Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350108, Fujian, Peoples R China
[2] Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
基金
中国国家自然科学基金;
关键词
high-resolution; leakage current; light-emitting diodes; nanoimprint; perovskite quantum dots; EFFICIENCY; MATRIX;
D O I
10.1002/adom.202202058
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Perovskite quantum dots (PQDs) have been widely used to realize light-emitting diodes (LEDs) with high color purity, efficiency, and wide color gamut. Due to the demand for huge amount of display information, development on high-resolution PQD LEDs (PQLEDs) with massive pixel density are highly desired. Herein, high-resolution PQLEDs are fabricated by using nanoimprint technique. By preparing a honeycomb-insulating polymer polymethyl methacrylate (PMMA) film, the high-resolution pixelated quantum dot emissive layer is formed. In addition, the leakage current of the device is significantly reduced because the direct contact between electron transport layer and hole transport layer is avoided. The PQLEDs based on nanoimprint technology show a resolution of 9072 pixels per inch (PPI), and a maximum external quantum efficiency (EQE) and brightness of 7.81% and 146 400 cd m(-2), respectively. The results demonstrate that high-resolution PQLEDs can be realized by using nanoimprint technology, holding great commercial potential for next-generation near-eye displays.
引用
收藏
页数:7
相关论文
共 38 条
[1]   25th Anniversary Article: Scalable Multiscale Patterned Structures Inspired by Nature: the Role of Hierarchy [J].
Bae, Won-Gyu ;
Kim, Hong Nam ;
Kim, Doogon ;
Park, Suk-Hee ;
Jeong, Hoon Eui ;
Suh, Kahp-Yang .
ADVANCED MATERIALS, 2014, 26 (05) :675-699
[2]   Surface Chemistry Engineering of Perovskite Quantum Dots: Strategies, Applications, and Perspectives [J].
Bai, Yang ;
Hao, Mengmeng ;
Ding, Shanshan ;
Chen, Peng ;
Wang, Lianzhou .
ADVANCED MATERIALS, 2022, 34 (04)
[3]   Flexible distributed feedback lasers based on nanoimprinted cellulose diacetate with efficient multiple wavelength lasing [J].
Castro Smirnov, Jose R. ;
Sousaraei, Ahmad ;
Osorio, Manuel R. ;
Casado, Santiago ;
Hernandez, Jaime J. ;
Wu, Longfei ;
Zhang, Qi ;
Xia, Ruidong ;
Granados, Daniel ;
Wannemacher, Reinhold ;
Rodriguez, Isabel ;
Cabanillas-Gonzalez, Juan .
NPJ FLEXIBLE ELECTRONICS, 2019, 3 (01)
[4]   Anion-exchange red perovskite quantum dots with ammonium iodine salts for highly efficient light-emitting devices [J].
Chiba, Takayuki ;
Hayashi, Yukihiro ;
Ebe, Hinako ;
Hoshi, Keigo ;
Sato, Jun ;
Sato, Shugo ;
Pu, Yong-Jin ;
Ohisa, Satoru ;
Kido, Junji .
NATURE PHOTONICS, 2018, 12 (11) :681-+
[5]   Wearable red-green-blue quantum dot light-emitting diode array using high-resolution intaglio transfer printing [J].
Choi, Moon Kee ;
Yang, Jiwoong ;
Kang, Kwanghun ;
Kim, Dong Chan ;
Choi, Changsoon ;
Park, Chaneui ;
Kim, Seok Joo ;
Chae, Sue In ;
Kim, Tae-Ho ;
Kim, Ji Hoon ;
Hyeon, Taeghwan ;
Kim, Dae-Hyeong .
NATURE COMMUNICATIONS, 2015, 6
[6]   Nanoimprint lithography [J].
Chou, SY ;
Krauss, PR ;
Renstrom, PJ .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 1996, 14 (06) :4129-4133
[7]   Perovskite QLED with an external quantum efficiency of over 21% by modulating electronic transport [J].
Fang, Tao ;
Wang, Tiantian ;
Li, Xiansheng ;
Dong, Yuhui ;
Bai, Sai ;
Song, Jizhong .
SCIENCE BULLETIN, 2021, 66 (01) :36-43
[8]   Lead Halide Perovskite Nanostructures for Dynamic Color Display [J].
Gao, Yisheng ;
Huang, Can ;
Hao, Chenglong ;
Sun, Shang ;
Zhang, Lei ;
Zhang, Chen ;
Duan, Zonghui ;
Wang, Kaiyang ;
Jin, Zhongwei ;
Zhang, Nan ;
Kildishev, Alexander, V ;
Qiu, Cheng-Wei ;
Song, Qinghai ;
Xiao, Shumin .
ACS NANO, 2018, 12 (09) :8847-8854
[9]   Nanoimprint Lithography Facilitated Plasmonic-Photonic Coupling for Enhanced Photoconductivity and Photocatalysis [J].
Gupta, Vaibhav ;
Sarkar, Swagato ;
Aftenieva, Olha ;
Tsuda, Takuya ;
Kumar, Labeesh ;
Schletz, Daniel ;
Schultz, Johannes ;
Kiriy, Anton ;
Fery, Andreas ;
Vogel, Nicolas ;
Koenig, Tobias A. F. .
ADVANCED FUNCTIONAL MATERIALS, 2021, 31 (36)
[10]   Patterning Multicolor Hybrid Perovskite Films via Top-Down Lithography [J].
Harwell, Jonathon ;
Burch, James ;
Fikouras, Alasdair ;
Gather, Malte C. ;
Di Falco, Andrea ;
Samuel, Ifor D. W. .
ACS NANO, 2019, 13 (04) :3823-3829