Characterisation of hydrogen jet flames under different pressures with varying coflow oxygen concentrations

被引:9
作者
Kildare, Jordan A. C. [1 ]
Evans, Michael J. [2 ]
Proud, Douglas B. [1 ]
Chin, Rey [1 ]
Tian, Zhao [1 ]
Medwell, Paul R. [1 ]
机构
[1] Univ Adelaide, Sch Elect & Mech Engn, Adelaide 5005, Australia
[2] Univ South Australia, UniSA STEM, Mawson Lakes 5095, Australia
基金
澳大利亚研究理事会;
关键词
Hydrogen combustion; MILD combustion; Jet flames; Pressure; Laminar flame calculations; DIRECT NUMERICAL-SIMULATION; MILD COMBUSTION; NOX-EMISSIONS; HEAT RELEASE; ASTERISK CHEMILUMINESCENCE; OH-ASTERISK; HOT; METHANE; AIR; DIFFUSION;
D O I
10.1016/j.ijhydene.2023.02.053
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The elevated temperature of hydrogen combustion increases the formation of thermal NOx. Moderate or intense low oxygen dilution (MILD) combustion is known to reduce NOx emissions and increase thermal efficiency. Pressure is often also used for increasing thermal efficiency. The impact that pressure has on fluid dynamics and chemical kinetics is especially relevant in MILD combustion conditions. Hydrogen jet flames issuing into a hot and vitiated coflow were imaged using OH* chemiluminescence at different pressures (1-7 bar) and oxygen levels (3-9% by vol.). Laminar flame simulations complemented the experiments. The observed mean radial OH* width increased with increased pressure, but only at O2 content less than 9%, suggesting that pressure has greater influence on kinetics when oxygen is reduced. The integrated OH* signal strength remained constant at 3% coflow O2, despite an apparent increase in flame width, suggesting a spatial broadening of the flame with pressure. Numerical results indicate that at 3-6% O2, conditions for MILD combustion of H2 are met across a wide range of strains and pressures, supporting the experimental observations for 3% O2.& COPY; 2023 The Author(s). Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC. This is an open access article under the CC BY license (http://creativecommons.org/ licenses/by/4.0/).
引用
收藏
页码:20059 / 20076
页数:18
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