Interface engineering for high-performance, triple-halide perovskite-silicon tandem solar cells

被引：265

作者：

Mariotti, Silvia ^{[1
,9
]}

Koehnen, Eike ^{[1
]}

Scheler, Florian ^{[1
]}

Sveinbjoernsson, Kari ^{[1
]}

Zimmermann, Lea ^{[1
]}

Piot, Manuel ^{[1
,2
]}

Yang, Fengjiu ^{[1
]}

Li, Bor ^{[1
]}

Warby, Jonathan ^{[3
]}

Musiienko, Artem ^{[1
]}

Menzel, Dorothee ^{[1
]}

Lang, Felix ^{[3
]}

Kessler, Sebastian ^{[1
]}

Levine, Igal ^{[1
]}

Mantione, Daniele ^{[4
,5
,6
]}

Al-Ashouri, Amran ^{[1
]}

Haertel, Marlene S. ^{[1
]}

Xu, Ke ^{[1
]}

Cruz, Alexandros ^{[1
]}

Kurpiers, Jona ^{[1
]}

Wagner, Philipp ^{[1
]}

Koebler, Hans ^{[1
]}

Li, Jinzhao ^{[1
]}

Magomedov, Artiom ^{[7
]}

Mecerreyes, David ^{[4
,6
]}

Unger, Eva ^{[1
]}

Abate, Antonio ^{[1
]}

Stolterfoht, Martin ^{[3
]}

Stannowski, Bernd ^{[1
]}

Schlatmann, Rutger ^{[1
]}

Korte, Lars ^{[1
]}

Albrecht, Steve ^{[1
,8
]}

机构：

[1] Helmholtz Zentrum Berlin Mat & Energie GmbH, Solar Energy Div, D-12489 Berlin, Germany

[2] Ecole Polytech Fed Lausanne, Inst Mat, Fac Engn, Lab Semicond Mat, CH-1015 Lausanne, Switzerland

[3] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany

[4] POLYKEY Polymers, Joxe Mari Korta Ctr, Donostia San Sebastian 20018, Spain

[5] Univ Basque Country UPV EHU, POLYMAT, Donostia San Sebastian 20018, Spain

[6] IKERBASQUE Basque Fdn Sci, Bilbao 48009, Spain

[7] Kaunas Univ Technol, Kaunas, Lithuania

[8] Tech Univ Berlin, Fak Elektrotech & Informat, D-10587 Berlin, Germany

[9] Okinawa Inst Sci & Technol Grad Univ OIST, Energy Mat & Surface Sci Unit EMSSU, Okinawa 9040495, Japan

来源：

SCIENCE | 2023年 / 381卷 / 6653期

关键词：

EFFICIENCY; PHOTOVOLTAICS;

D O I：

10.1126/science.adf5872

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

Improved stability and efficiency of two-terminal monolithic perovskite-silicon tandem solar cells will require reductions in recombination losses. By combining a triple-halide perovskite (1.68 electron volt bandgap) with a piperazinium iodide interfacial modification, we improved the band alignment, reduced nonradiative recombination losses, and enhanced charge extraction at the electron-selective contact. Solar cells showed open-circuit voltages of up to 1.28 volts in p-i-n single junctions and 2.00 volts in perovskite-silicon tandem solar cells. The tandem cells achieve certified power conversion efficiencies of up to 32.5%.

引用

页码：63 / 69

页数：7

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