Full-dimensional quantum mechanical study of three-body recombination for cold 4He-4He-20Ne system

被引:2
作者
Zhao, Ming-Ming [1 ]
Wang, Bin-Bin [2 ]
Wang, Gao-Ren [1 ,3 ]
Fu, Bina [4 ]
Shundalau, Maksim [3 ,5 ,6 ]
Han, Yong-Chang [1 ,3 ]
机构
[1] Dalian Univ Technol, Dept Phys, Dalian 116024, Peoples R China
[2] China West Normal Univ, Sch Phys & Astron, Nanchong 637009, Peoples R China
[3] Dalian Univ Technol, DUT BSU Joint Inst, Dalian 116024, Peoples R China
[4] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
[5] Belarusian State Univ, Phys Dept, Minsk, BELARUS
[6] Univ Salerno, Dept Informat Engn & Elect & Appl Math, DIEM, , SA, Fisciano, Italy
基金
中国国家自然科学基金; 国家重点研发计划;
关键词
COLLISION-INDUCED DISSOCIATION; MAGNETIC-FIELD DEPENDENCE; INELASTIC-COLLISIONS; FESHBACH RESONANCES; DYNAMICS; ENERGY; STATES; ATOMS; GAS;
D O I
10.1063/5.0144619
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The increase of the number of the two-body recombination channels strongly challenges the numerical calculation of the accurate rates for the three-body recombination (TBR) process and its reverse process, collision-induced dissociation (CID), at ultracold temperatures. By taking the He-4-He-4-Ne-20 collision system as an example, we have obtained the rates for its TBR and CID processes involving all four recombination channels, including the two-body states He-4(2) (l = 0) and (HeNe)-He-4-Ne-20 (l = 0, 1, 2) with l the rotational quantum number. By using the adiabatic hyperspherical method, we have considered not only total angular momentum J = 0 but also J > 0 in the ultracold collision energies (E = 0.01 - 100 mK x k(B)). It is found that He-4(2) (l = 0) is the major product after the TBR process in the ultracold limit (E = 0.1 mK x k(B)). The TBR rate into He-4(2) (l = 0) is nearly one order of magnitude larger than the sum of the other three products, (HeNe)-He-4-Ne-20 (l = 0, 1, 2). Moreover, the CID rates for the three (HeNe)-He-4-Ne-20 (l = 0, 1, 2) + He-4 initial states are close to each other and are smaller than that for the He-4(2) (l = 0) + Ne-20 initial state. Additionally, we have, for the first time, performed the channel-resolved scattering calculation that can explain the above-mentioned findings quantitatively.
引用
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页数:11
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