Electrochemical scanning probe microscopies for artificial photosynthesis

被引：5
作者：
Yang, Chunlei [1 ,2 ]
Su, Tianhui [1 ,2 ]
Hua, Yanbo [1 ,2 ]
Zhang, Liming [1 ,2 ]
机构：
[1] Fudan Univ, iChEM Collaborat Innovat Ctr Chem Energy Mat, Dept Chem, Shanghai 200438, Peoples R China
[2] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200438, Peoples R China
来源：
NANO RESEARCH | 2023年 / 16卷 / 03期
基金：
中国国家自然科学基金;
关键词：
(photo)electrocatalysis; scanning probe microscopies; scanning tunneling microscopy; atomic force microscopy; in-situ; ATOMIC-FORCE MICROSCOPY; OXYGEN EVOLUTION; CHARGE SEPARATION; WATER OXIDATION; SURFACE INTERROGATION; ELECTRIC-FIELDS; DOUBLE-LAYER; INTERFACES; CATALYSTS; PHOTOCATALYST;
D O I：
10.1007/s12274-022-5326-y
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The rational design of efficient artificial photosynthetic components requires thorough understandings towards (photo)electrochemical properties and kinetic processes at the solid/liquid interface. Electrochemical scanning probe microscopy (EC-SPM), which enables the high-spatial resolution imaging in an electrolyte environment, becomes an indispensable experimental technique for operando studies of (photo)electrochemistry. This review summarizes the latest results of relevant EC-SPM techniques to study the interfacial properties of electrocatalysts and photoelectrodes. Covered methods include atomic force microscopy, Kelvin probe force microscopy, conductive atomic force microscopy, scanning tunneling microscopy, scanning electrochemical microscopy, and other advanced SPM-based operando techniques. Finally, we offer some perspectives on the future outlook in this fascinating research area.
引用
收藏
页码：4013 / 4028
页数：16
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