Nanographene-Based Heterojunctions for High-Performance Organic Phototransistor Memory Devices

被引:29
作者
Bai, Shaoling [1 ,2 ]
Yang, Lin [1 ,3 ]
Haase, Katherina [1 ,2 ]
Wolansky, Jakob [4 ,5 ]
Zhang, Zongbao [4 ,5 ]
Tseng, Hsin [4 ,5 ]
Talnack, Felix [1 ,2 ]
Kress, Joshua [4 ,5 ]
Andrade, Jonathan Perez [1 ,2 ,6 ]
Benduhn, Johannes [4 ,5 ]
Ma, Ji [1 ,3 ,7 ]
Feng, Xinliang [1 ,3 ,7 ]
Hambsch, Mike
Mannsfeld, Stefan C. B. [2 ]
机构
[1] Tech Univ Dresden, Ctr Adv Elect Dresden Cfaed, Helmholtzstr 18, D-01062 Dresden, Germany
[2] Tech Univ Dresden, Fac Elect & Comp Engn, Helmholtzstr 18, D-01062 Dresden, Germany
[3] Tech Univ Dresden, Fac Chem & Food Chem, Helmholtzstr 18, D-01062 Dresden, Germany
[4] Tech Univ Dresden, Dresden Integrated Ctr Appl Phys & Photon Mat IAPP, Nothnitzer Str 61, D-01187 Dresden, Germany
[5] Tech Univ Dresden, Inst Appl Phys, Nothnitzer Str 61, D-01187 Dresden, Germany
[6] Leibniz Inst Solid State & Mat Res, Helmholtzstr 20, D-01069 Dresden, Germany
[7] Max Planck Inst Microstruct Phys, Weinberg 2, D-06120 Halle, Germany
基金
欧盟地平线“2020”;
关键词
memory; nanographene; organic phototransistors; photosensitivity; ELECTRON-MOBILITY TRANSISTORS; HYDROCARBONS; DETECTORS;
D O I
10.1002/advs.202300057
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Organic phototransistors can enable many important applications such as nonvolatile memory, artificial synapses, and photodetectors in next-generation optical communication and wearable electronics. However, it is still a challenge to achieve a big memory window (threshold voltage response increment V-th) for phototransistors. Here, a nanographene-based heterojunction phototransistor memory with large increment V-th responses is reported. Exposure to low intensity light (25.7 mu W cm(-2)) for 1 s yields a memory window of 35 V, and the threshold voltage shift is found to be larger than 140 V under continuous light illumination. The device exhibits both good photosensitivity (3.6 x 10(5)) and memory properties including long retention time (>1.5 x 10(5) s), large hysteresis (45.35 V), and high endurance for voltage-erasing and light-programming. These findings demonstrate the high application potential of nanographenes in the field of optoelectronics. In addition, the working principle of these hybrid nanographene-organic structured heterojunction phototransistor memory devices is described which provides new insight into the design of high-performance organic phototransistor devices.
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页数:12
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