Activated carbon cloth electrodes for capacitive deionization: a neutron imaging study

被引:0
|
作者
Butcher, Tim A. [1 ,2 ,7 ]
Prendeville, Lucy [1 ,2 ]
Rafferty, Aran [3 ,4 ]
Trtik, Pavel [5 ]
Boillat, Pierre [5 ,6 ]
Coey, J. M. D. [1 ,2 ]
机构
[1] Trinity Coll Dublin, Sch Phys, Dublin, Ireland
[2] Trinity Coll Dublin, CRANN, Dublin, Ireland
[3] Trinity Coll Dublin, AMBER Res Ctr, Dublin, Ireland
[4] Trinity Coll Dublin, Sch Chem, Dublin, Ireland
[5] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland
[6] Paul Scherrer Inst PSI, Electrochem Lab, Villigen, Switzerland
[7] Paul Scherrer Inst, Lab Condensed Matter, CH-5232 Villigen, Switzerland
来源
基金
欧盟地平线“2020”;
关键词
Activated carbon; Desalination; Electrosorption; Ion transport; Micropores; Neutron imaging; SMALL-ANGLE NEUTRON; DENSITY-FUNCTIONAL THEORY; WATER DESALINATION; MICROPOROUS CARBON; CHARGE EFFICIENCY; PORE-SIZE; SCATTERING; ELECTROSORPTION; ADSORPTION; TRANSPORT;
D O I
10.1007/s00339-024-07343-8
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Neutron imaging was employed to track the uptake of Gd3+\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$<^>{3+}$$\end{document} ions by the sub 2 nm micropores of charged activated carbon cloth electrodes from an aqueous Gd(NO3\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$_3$$\end{document})3\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$_3$$\end{document} solution. The transmitted neutron intensity evinces the persistent presence of Gd3+\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$<^>{3+}$$\end{document} in the micropores during the discharge cycle, which is caused by the adsorption of oppositely charged ions. The charge efficiency of the activated carbon cloth system was determined by direct comparison with the imaged Gd3+\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$<^>{3+}$$\end{document} concentration changes, with which the influence of ion swapping and resistive losses on capacitive deionization cells can be ascertained.
引用
收藏
页数:9
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