Novel high-efficient adsorbent based on modified gelatin/montmorillonite nanocomposite for removal of malachite green dye

被引:23
|
作者
Abu Elella, Mahmoud H. [1 ]
Aamer, Nema [1 ]
Abdallah, Heba M. [2 ]
Lopez-Maldonado, Eduardo A. [3 ]
Mohamed, Yasser M. A. [4 ]
El Nazer, Hossam A. [4 ]
Mohamed, Riham R. [1 ]
机构
[1] Cairo Univ, Fac Sci, Chem Dept, Giza 12613, Egypt
[2] Natl Res Ctr, Chem Ind Res Inst, Polymers & Pigments Dept, Giza 12622, Egypt
[3] Autonomous Univ Baja California, Fac Chem Sci & Engn, Tijuana 22390, Baja California, Mexico
[4] Natl Res Ctr, Photochem Dept, Giza 12622, Egypt
关键词
HEAVY-METAL IONS; AQUEOUS-SOLUTION; METHYLENE-BLUE; HYBRID NANOCOMPOSITE; MONTMORILLONITE CLAY; OXYGEN BARRIER; ACRYLIC-ACID; XANTHAN GUM; ADSORPTION; GELATIN;
D O I
10.1038/s41598-024-51321-2
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Shortage of drinking water has gained potential interest over the last few decades. Discharged industrial effluent, including various toxic pollutants, to water surfaces is one of the most serious environmental issues. The adsorption technique has become a widely studied method for the removal of toxic pollutants, specifically synthetic dyes, from wastewater due to its cost-effectiveness, high selectivity, and ease of operation. In this study, a novel gelatin-crosslinked-poly(acrylamide-co-itaconic acid)/montmorillonite (MMT) nanoclay nanocomposites-based adsorbent has been prepared for removing malachite green (MG) dye from an aqueous solution. Modified gelatin nanocomposites were synthesized using a free-radical polymerization technique in the presence and absence of MMT. Various analytical instrumentation: including FTIR, FESEM, XRD, and TEM techniques were used to elucidate the chemical structure and surface morphology of the prepared samples. Using a batch adsorption experiment, Langmuir isotherm model showed that the prepared modified gelatin nanocomposite had a maximum adsorption capacity of 950.5 mg/g using 350 mg/L of MG dye at pH 9 within 45 min. Furthermore, the regeneration study showed good recyclability for the obtained nanocomposite through four consecutive reusable cycles. Therefore, the fabricated gelatin nanocomposite is an attractive adsorbent for MG dye elimination from aqueous solutions.
引用
收藏
页数:15
相关论文
共 50 条
  • [31] Xerogel activated diatoms as an effective hybrid adsorbent for the efficient removal of malachite green
    Sriram, Ganesan
    Uthappa, U. T.
    Kigga, Madhuprasad
    Jung, Ho-Young
    Altalhi, Tariq
    Brahmkhatri, Varsha
    Kurkuri, Mahaveer D.
    NEW JOURNAL OF CHEMISTRY, 2019, 43 (09) : 3810 - 3820
  • [32] Novel hydrogel based on natural hybrid backbones: optimized synthesis and effective adsorbent for the removal of malachite green dye from an aqueous solution
    Kumawat, Yogesh Kumar
    Nair, Abhigith
    Choudhary, Sonal
    Nath, Jyotendra
    Sharma, Kashma
    Rasool, Tanveer
    Sharma, Vishal
    Mishra, Yogendra Kumar
    Kumar, Vijay
    JOURNAL OF POLYMER RESEARCH, 2024, 31 (05)
  • [33] Amino ionic liquids-modified magnetic core/shell nanocomposite as an efficient adsorbent for dye removal
    Cheng, Jingjing
    Shi, Lijuan
    Lu, Jianjun
    JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2016, 36 : 206 - 214
  • [34] Magnetic nanocellulose-based adsorbent for highly selective removal of malachite green from mixed dye solution
    Zhang, Xuelun
    Qiu, Chongpeng
    Li, Feng
    Zhang, Xuefeng
    Li, Mei-Chun
    Xie, Jiulong
    de Hoop, Cornelis F.
    Qi, Jinqiu
    Huang, Xingyan
    INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES, 2023, 253
  • [35] Removal of malachite green using carboxymethyl cellulose-g- polyacrylamide/montmorillonite nanocomposite hydrogel
    Peighambardoust, Seyed Jamaleddin
    Aghamohammadi-Bavil, Omid
    Foroutan, Rauf
    Arsalani, Nasser
    INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES, 2020, 159 : 1122 - 1131
  • [36] Investigation on removal of malachite green using EM based compost as adsorbent
    Pushpa, T. Bhagavathi
    Vijayaraghavan, J.
    Basha, S. J. Sardhar
    Sekaran, V.
    Vijayaraghavan, K.
    Jegan, J.
    ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY, 2015, 118 : 177 - 182
  • [37] Adsorption of malachite green on the modified montmorillonite/xanthan gum-sodium alginate hybrid nanocomposite
    Rahmani, Mehdi
    Koohi, Ahmad Dadvand
    POLYMER BULLETIN, 2022, 79 (10) : 8241 - 8267
  • [38] Removal of toxic malachite green dye from aqueous environment using reduced magnetic graphene oxide as an efficient and reusable adsorbent
    Gul, Kashif
    Khan, Hamayun
    Muhammad, Niaz
    Ara, Behisht
    Zia, Tanveer Ul Haq
    SEPARATION SCIENCE AND TECHNOLOGY, 2021, 56 (15) : 2507 - 2520
  • [39] Adsorption of malachite green on the modified montmorillonite/xanthan gum-sodium alginate hybrid nanocomposite
    Mehdi Rahmani
    Ahmad Dadvand Koohi
    Polymer Bulletin, 2022, 79 : 8241 - 8267
  • [40] Synthesis of Datura inoxia-added iron nanoparticle adsorbent for malachite green dye removal
    Sharma, Y.
    Bhateria, R.
    INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY, 2024, 21 (04) : 3689 - 3704