Giant Exchange-Bias-Like Effect at Low Cooling Fields Induced by Pinned Magnetic Domains in Y2NiIrO6 Double Perovskite

被引:66
作者
Deng, Zheng [1 ,2 ]
Wang, Xiao [3 ]
Wang, Mengqin [1 ]
Shen, Feiran [4 ]
Zhang, Jine [1 ]
Chen, Yuansha [1 ]
Feng, Hai L. L. [1 ]
Xu, Jiawang [1 ]
Peng, Yi [1 ]
Li, Wenmin [1 ]
Zhao, Jianfa [1 ]
Wang, Xiancheng [1 ]
Valvidares, Manuel [5 ]
Francoual, Sonia [6 ]
Leupold, Olaf [6 ]
Hu, Zhiwei [3 ]
Tjeng, Liu Hao [3 ]
Li, Man-Rong [7 ]
Croft, Mark [8 ]
Zhang, Ying [1 ]
Liu, Enke [1 ]
He, Lunhua [1 ,9 ]
Hu, Fengxia [1 ]
Sun, Jirong [1 ]
Greenblatt, Martha [2 ]
Jin, Changqing [1 ]
机构
[1] Chinese Acad Sci, Univ Chinese Acad Sci, Inst Phys, Sch Phys, Beijing 100190, Peoples R China
[2] Rutgers State Univ, Dept Chem & Chem Biol, 123 Bevier Rd, Piscataway, NJ 08854 USA
[3] Max Planck Inst Chem Phys Solids, Nothnitzer Str 40, D-01187 Dresden, Germany
[4] Chinese Acad Sci, Inst High Energy Phys, Spallat Neutron Source Sci Ctr, Dongguan 523803, Peoples R China
[5] ALBA Synchrotron Light Source, Barcelona 08290, Spain
[6] Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany
[7] Sun Yat Sen Univ, Sch Chem, Key Lab Bioinorgan & Synthet Chem, Minist Educ, Guangzhou 510275, Peoples R China
[8] Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA
[9] Spallat Neutron Source Sci Ctr, Songshan Lake Mat Lab, Dongguan 523808, Peoples R China
关键词
cooling field; double perovskite; magnetic domain; single-phase material; spin-orbit coupling; RAY CIRCULAR-DICHROISM; ELECTRIC CONTROL; DESIGN;
D O I
10.1002/adma.202209759
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Exchange bias (EB) is highly desirable for widespread technologies. Generally, conventional exchange-bias heterojunctions require excessively large cooling fields for sufficient bias fields, which are generated by pinned spins at the interface of ferromagnetic and antiferromagnetic layers. It is crucial for applicability to obtain considerable exchange-bias fields with minimum cooling fields. Here, an exchange-bias-like effect is reported in a double perovskite, Y2NiIrO6, which shows long-range ferrimagnetic ordering below 192 K. It displays a giant bias-like field of 1.1 T with a cooling field of only 15 Oe at 5 K. This robust phenomenon appears below 170 K. This fascinating bias-like effect is the secondary effect of the vertical shifts of the magnetic loops, which is attributed to the pinned magnetic domains due to the combination of strong spin-orbit coupling on Ir, and antiferromagnetically coupled Ni- and Ir-sublattices. The pinned moments in Y2NiIrO6 are present throughout the full volume, not just at the interface as in conventional bilayer systems.
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页数:8
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