Composite magnetic sorbents based on magnetic Fe3O4 coated by Zn and Al layered double hydroxide for U(VI) removal from aqueous media

被引：15
|
作者：
Ivanov, N. P. [1 ]
Dran'kov, A. N. [1 ]
Shichalin, O. O. [1 ]
Lembikov, A. O. [1 ]
Buravlev, I. Yu. [1 ]
Mayorov, V. Yu. [1 ]
Balanov, M. I. [1 ]
Rogachev, K. A. [1 ]
Kaspruk, G. D. [1 ]
Pisarev, S. M. [1 ]
Marmaza, P. A. [1 ]
Rastorguev, V. L. [1 ]
Balybina, V. A. [1 ]
Fedorets, A. N. [1 ]
Kaptakov, V. O. [2 ]
Papynov, E. K. [1 ]
机构：
[1] Far Eastern Fed Univ, 10 Ajax Bay, Vladivostok 690922, Russia
[2] Russian Acad Sci, Inst Phys Chem & Electrochem, Bld 4,31 Leninsky Prospect, Moscow 119072, Russia
来源：
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY | 2024年 / 333卷 / 03期
关键词：
Uranium; Sorbent; Layered double hydroxides; Magnetic composite materials; Adsorption; EFFICIENT REMOVAL; URANIUM; IONS; SORPTION; POLYETHYLENIMINE; NANOCOMPOSITE; NANOPARTICLES; EXTRACTION; RECOVERY; OXIDES;
D O I：
10.1007/s10967-024-09362-4
中图分类号：
O65 [分析化学];
学科分类号：
070302 ; 081704 ;
摘要：
Composite sorbents based on Fe3O4 and Zn-Al-LDH with different weight ratios of magnetic and sorbing phases were obtained by the precipitation method. The optimal weight ratio of Zn/Fe was 16, which resulted in a 62% increase in hydromechanical strength. The maximum sorption exchange capacity towards U(VI) was 268.65 +/- 22.22 mg/g. The efficiency of U(VI) adsorption was not affected by the presence of Cl-, SO42-, NO3- and Na+, Ca2+. The distribution coefficient in a groundwater model solution was K-d(U(VI) = 0.5-3 x 10(5) mL/g. The materials possess high exchange capacity and selectivity, which makes them suitable sorbents for U(VI) removal.
引用
收藏
页码：1213 / 1230
页数：18
相关论文
共 50 条
  • [21] Highly efficient removal of Cr(VI) from wastewater via adsorption with novel magnetic Fe3O4@C@MgAl-layered double-hydroxide
    Zhang, Hui
    Huang, Fei
    Liu, De-Lei
    Shi, Peng
    CHINESE CHEMICAL LETTERS, 2015, 26 (09) : 1137 - 1143
  • [22] Preparation of Fe3O4@C@Layered Double Hydroxide Composite for Magnetic Separation of Uranium
    Zhang, Xiaofei
    Wang, Jun
    Li, Rumin
    Dai, Qihui
    Gao, Rui
    Liu, Qi
    Zhang, Milin
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2013, 52 (30) : 10152 - 10159
  • [23] Magnetic Sorbents for Removing U(VI) from Aqueous Media
    Puzyrnaya L.N.
    Shunkov V.S.
    Pshinko G.N.
    Kosorukov A.A.
    Radiochemistry, 2018, 60 (03) : 281 - 286
  • [24] Efficient removal of iodide anion from aqueous solution with recyclable core-shell magnetic Fe3O4 @Mg/Al layered double hydroxide (LDH)
    Jung, Il-Kwon
    Jo, Yongheum
    Han, Sol-Chan
    Yun, Jong-Il
    SCIENCE OF THE TOTAL ENVIRONMENT, 2020, 705 (705)
  • [25] Synthesis of magnetic nanocomposite Fe3O4 coated polypyrrole (PPy) for Chromium(VI) removal
    Mirrezaie, Najme
    Nikazar, Manochehr
    Zadeh, Mehrdad Hasan
    ULTRAFINE GRAINED AND NANO-STRUCTURED MATERIALS IV, 2014, 829 : 649 - 653
  • [26] Surface mercapto engineered magnetic Fe3O4 nanoadsorbent for the removal of mercury from aqueous solutions
    Pan, Shengdong
    Shen, Haoyu
    Xu, Qihong
    Luo, Jian
    Hu, Meiqin
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2012, 365 (01) : 204 - 212
  • [27] Removal of fluoride from aqueous solution by polypyrrole/Fe3O4 magnetic nanocomposite
    Bhaumik, Madhumita
    Leswifi, Taile Yvonne
    Maity, Arjun
    Srinivasu, V. V.
    Onyango, Maurice S.
    JOURNAL OF HAZARDOUS MATERIALS, 2011, 186 (01) : 150 - 159
  • [28] Facile synthesis of magnetic Fe3O4/graphene composites for enhanced U(VI) sorption
    Zhao, Donglin
    Zhu, Hongyu
    Wu, Changnian
    Feng, Shaojie
    Alsaedi, Ahmed
    Hayat, Tasawar
    Chen, Changlun
    APPLIED SURFACE SCIENCE, 2018, 444 : 691 - 698
  • [29] Adsorption of U(VI) from aqueous solution by magnetic core-dual shell Fe3O4@PDA@TiO2
    Zhang, Hui
    Dai, Zhongran
    Sui, Yang
    Xue, Jinhua
    Ding, Dexin
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2018, 317 (01) : 613 - 624
  • [30] Fabrication of Magnetic Fe/Zn Layered Double Oxide@Carbon Nanotube Composites and Their Application for U(VI) and 241Am(III) Removal
    Chen, Haijun
    Zhang, Zhibin
    Wang, Xiangxue
    Chen, Jing
    Xu, Chao
    Liu, Yunhai
    Yu, Zhimin
    Wang, Xiangke
    ACS APPLIED NANO MATERIALS, 2018, 1 (05): : 2386 - 2396
12345