Fabrication of nanoconfined spaces of KIT-6 with small-sized SnO2 for enhanced oxidative desulfurization of fuel: Kinetics and thermodynamics
被引:12
作者:
Ahmad, Mateen
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China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R ChinaChina Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Ahmad, Mateen
[1
]
Zhen, Liu
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China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R ChinaChina Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Zhen, Liu
[1
]
Aslam, Sobia
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China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Abdul Wali Khan Univ Mardan, Dept Chem, Mardan, PakistanChina Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Aslam, Sobia
[1
,2
]
Subhan, Fazle
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China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Abdul Wali Khan Univ Mardan, Dept Chem, Mardan, PakistanChina Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Subhan, Fazle
[1
,2
]
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Ullah, Hameed
[2
]
Yan, Zifeng
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China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R ChinaChina Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
Yan, Zifeng
[1
]
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Zada, Amir
[2
]
机构:
[1] China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China
[2] Abdul Wali Khan Univ Mardan, Dept Chem, Mardan, Pakistan
SnO2 functionalized catalysts have great potential in oxidative desulfurization (ODS) of fuels. However, a facile strategy is required to enhance its catalytic performance. In this contribution, solid phase grinding (SPG) strategy is proposed to functionalize as-synthesized KIT-6 (AK-6) with SnO2 NPs. The SnCl2<middle dot>2H(2)O was directly incorporated into the confined spaces between silica walls and template of AK-6 and the subsequent calcination not only remove template (P123) but also convert SnCl2<middle dot>2H(2)O to SnO2, which saves much time and energy. Confined spaces and silanols of AK-6 regulated the size and dispersion of SnO2 NPs up to loading of 10 wt% SnO2 (Sn10AK-6). In contrast, larger SnO2 NPs were observed in Sn10CK-6 derived from calcined KIT-6 (CK-6). The activity of Sn10AK-6 is also higher than Sn10CK-6 and converts 96.5 % DBT to sulfones at 303 K in 40 min with 0.1 g of catalyst using O/S = 4 M ratio of NaOCl. The DBT conversion over Sn10AK-6/NaOCl followed pseudo first order kinetics. Moreover, the calculated activation energy of 46.08 kJ/mol and thermodynamic parameters like Delta H = 49.70 kJ/mol, Delta S = -437 J/mol K and Delta G = 180.30 kJ/mol evinced that the ODS over Sn10AK-6 is endergonic, non-spontaneous and practicable under ambient conditions.
机构:
Zentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Optenhostert, Thomas
Puthenkalam, Sissy
论文数: 0引用数: 0
h-index: 0
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Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Puthenkalam, Sissy
Stegmann, Niklas
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Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Stegmann, Niklas
Steffen, Michael
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Zentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Steffen, Michael
Schmidt, Wolfgang
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Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
机构:
Univ Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Univ Indonesia, Integrated Lab Energy & Environm, Fak MIPA, Depok 16424, IndonesiaUniv Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Paramarta, V.
Taufik, A.
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Univ Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Univ Indonesia, Integrated Lab Energy & Environm, Fak MIPA, Depok 16424, IndonesiaUniv Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Taufik, A.
Saleh, R.
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Univ Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Univ Indonesia, Integrated Lab Energy & Environm, Fak MIPA, Depok 16424, IndonesiaUniv Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Saleh, R.
[J].
8TH INTERNATIONAL CONFERENCE ON PHYSICS AND ITS APPLICATIONS (ICOPIA),
2016,
776
机构:
DCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Deenbandhu Chhotu Ram Univ Sci Technol, Phys Chem Res Lab, Dept Chem, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Poonia, Ekta
Dahiya, Manjeet S.
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DCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Dahiya, Manjeet S.
Tomer, Vijay K.
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Inst Mat Sci Agh, Synth & Real Struct Grp, CAU, D-24143 Kiel, GermanyDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Tomer, Vijay K.
Kumar, Krishan
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Deenbandhu Chhotu Ram Univ Sci Technol, Phys Chem Res Lab, Dept Chem, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Kumar, Krishan
Kumar, Sunil
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Indian Inst Technol, Discipline Met Engn & Mat Sci, Indore 453552, Simrol, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Kumar, Sunil
Duhan, Surender
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DCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Rajendran, Antony
Cui, Tian-you
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Cui, Tian-you
Fan, Hong-xia
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Fan, Hong-xia
Yang, Zhi-fen
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Yang, Zhi-fen
Feng, Jie
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Feng, Jie
Li, Wen-ying
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Ren, Xiaoling
Miao, Guang
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机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Miao, Guang
Xiao, Zhiyong
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Xiao, Zhiyong
Ye, Feiyan
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Ye, Feiyan
Li, Zhong
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机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Li, Zhong
Wang, Haihui
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机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Wang, Haihui
Xiao, Jing
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S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R ChinaS China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
机构:
Zentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Optenhostert, Thomas
Puthenkalam, Sissy
论文数: 0引用数: 0
h-index: 0
机构:
Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Puthenkalam, Sissy
Stegmann, Niklas
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h-index: 0
机构:
Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Stegmann, Niklas
Steffen, Michael
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Zentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
Steffen, Michael
Schmidt, Wolfgang
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h-index: 0
机构:
Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, GermanyZentrum Brennstoffzellentech GmbH, Carl Benz Str 201, D-47057 Duisburg, Germany
机构:
Univ Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Univ Indonesia, Integrated Lab Energy & Environm, Fak MIPA, Depok 16424, IndonesiaUniv Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Paramarta, V.
Taufik, A.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Univ Indonesia, Integrated Lab Energy & Environm, Fak MIPA, Depok 16424, IndonesiaUniv Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Taufik, A.
Saleh, R.
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h-index: 0
机构:
Univ Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Univ Indonesia, Integrated Lab Energy & Environm, Fak MIPA, Depok 16424, IndonesiaUniv Indonesia, Dept Fis, Fak MIPA, Depok 16424, Indonesia
Saleh, R.
[J].
8TH INTERNATIONAL CONFERENCE ON PHYSICS AND ITS APPLICATIONS (ICOPIA),
2016,
776
机构:
DCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Deenbandhu Chhotu Ram Univ Sci Technol, Phys Chem Res Lab, Dept Chem, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Poonia, Ekta
Dahiya, Manjeet S.
论文数: 0引用数: 0
h-index: 0
机构:
DCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Dahiya, Manjeet S.
Tomer, Vijay K.
论文数: 0引用数: 0
h-index: 0
机构:
Inst Mat Sci Agh, Synth & Real Struct Grp, CAU, D-24143 Kiel, GermanyDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Tomer, Vijay K.
Kumar, Krishan
论文数: 0引用数: 0
h-index: 0
机构:
Deenbandhu Chhotu Ram Univ Sci Technol, Phys Chem Res Lab, Dept Chem, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Kumar, Krishan
Kumar, Sunil
论文数: 0引用数: 0
h-index: 0
机构:
Indian Inst Technol, Discipline Met Engn & Mat Sci, Indore 453552, Simrol, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
Kumar, Sunil
Duhan, Surender
论文数: 0引用数: 0
h-index: 0
机构:
DCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, IndiaDCR Univ Sci & Technol, Dept Mat Sci & Nanotechnol, Nanomat Res Lab, Murthal 131039, Haryana, India
机构:
Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Rajendran, Antony
Cui, Tian-you
论文数: 0引用数: 0
h-index: 0
机构:
Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Cui, Tian-you
Fan, Hong-xia
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h-index: 0
机构:
Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Fan, Hong-xia
Yang, Zhi-fen
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h-index: 0
机构:
Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Yang, Zhi-fen
Feng, Jie
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h-index: 0
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Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
Feng, Jie
Li, Wen-ying
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h-index: 0
机构:
Taiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R ChinaTaiyuan Univ Technol, Training Base State Key Lab Coal Sci & Technol Jo, Minist Sci & Technol, Taiyuan 030024, Peoples R China
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Ren, Xiaoling
Miao, Guang
论文数: 0引用数: 0
h-index: 0
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Miao, Guang
Xiao, Zhiyong
论文数: 0引用数: 0
h-index: 0
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Xiao, Zhiyong
Ye, Feiyan
论文数: 0引用数: 0
h-index: 0
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Ye, Feiyan
Li, Zhong
论文数: 0引用数: 0
h-index: 0
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Li, Zhong
Wang, Haihui
论文数: 0引用数: 0
h-index: 0
机构:S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Wang, Haihui
Xiao, Jing
论文数: 0引用数: 0
h-index: 0
机构:
S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R ChinaS China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China