Zeolitic-imidazolate-framework-derived Fe-NC catalysts towards efficient oxygen reduction reaction

被引：7
作者：
Ren, Jingru [1 ]
Shi, Zihan [1 ]
Huang, Yongmin [1 ]
机构：
[1] East China Univ Sci & Technol, Sch Chem & Mol Engn, Related Technol Minist Educ, Key Lab Specially Funct Polymer Mat & Related Tech, Shanghai 200237, Peoples R China
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2023年 / 48卷 / 33期
关键词：
ZIF-8; M-N-C; Electrocatalyst; Oxygen reduction reaction; NITROGEN-DOPED GRAPHENE; HIGH-PERFORMANCE; FUEL-CELLS; CATHODE CATALYST; ORR CATALYST; CARBON; ELECTROCATALYST; NANOPARTICLES; STRATEGY; DESIGN;
D O I：
10.1016/j.ijhydene.2022.12.099
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The development of non-precious metal catalysts to replace scarce and expensive Pt-based catalysts is critical for oxygen reduction reactions (ORR), where zeolitic-imidazolate-framework-derived (ZIF-derived) iron-based electrocatalysts hold a promising prospect. Herein, Fe3O4 was used as Fe source, and ZIF-8 was used as C and N source to prepare Fe-NC catalysts. Specifically, the half-wave potential (E1/2) of the Fe-NC reached 0.90 V, which was higher than commercial Pt/C catalysts (0.87 V), and the overpotential of OER reached 327 mV. In addition, the power density tested in Zn-air batteries upped to 129.59 mW cm-2, surpassing that of the Pt/C (108.93 mW cm-2). The superior performance was attributed to the effective introduction of Fe, the large specific surface area (851.6 m2 g-1), relatively regular porous structure and the high degree of graphitization. (c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：12333 / 12341
页数：9
相关论文
共 57 条
[1]   A quick guide to the assessment of key electrochemical performance indicators for the oxygen reduction reaction: A comprehensive review [J].
Bhuvanendran, Narayanamoorthy ;
Ravichandran, Sabarinathan ;
Xu, Qian ;
Maiyalagan, Thandavarayan ;
Su, Huaneng .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (11) :7113-7138
[2]   Best practices for ORR performance evaluation of metal-free porous carbon electrocatalysts [J].
Bouleau, L. ;
Perez-Rodriguez, S. ;
Quilez-Bermejo, J. ;
Izquierdo, M. T. ;
Xu, F. ;
Fierro, V. ;
Celzard, A. .
CARBON, 2022, 189 :349-361
[3]   Oxygen Reduction Electrocatalysis with Epitaxially Grown Spinel MnFe2O4 and Fe3O4 [J].
Bredar, Alexandria R. C. ;
Blanchet, Miles D. ;
Burton, Andricus R. ;
Matthews, Bethany E. ;
Spurgeon, Steven R. ;
Comes, Ryan B. ;
Farnum, Byron H. .
ACS CATALYSIS, 2022, 12 (06) :3577-3588
[4]   Advanced Exfoliation Strategies for Layered Double Hydroxides and Applications in Energy Conversion and Storage [J].
Chen, Chen ;
Tao, Li ;
Du, Shiqian ;
Chen, Wei ;
Wang, Yanyong ;
Zou, Yuqin ;
Wang, Shuangyin .
ADVANCED FUNCTIONAL MATERIALS, 2020, 30 (14)
[5]   Hypercrosslinked polymer-mediated fabrication of binary metal phosphide decorated spherical carbon as an efficient and durable bifunctional electrocatalyst for rechargeable Zn-air batteries [J].
Chen, Haowen ;
Liu, Yijiang ;
Liu, Bei ;
Yang, Mei ;
Li, Huaming ;
Chen, Hongbiao .
NANOSCALE, 2022, 14 (34) :12431-12436
[6]   Iron-incorporated nitrogen-doped carbon materials as oxygen reduction electrocatalysts for zinc-air batteries [J].
Chen, Kai ;
Ci, Suqin ;
Xu, Qiuhua ;
Cai, Pingwei ;
Li, Meizhen ;
Xiang, Lijuan ;
Hu, Xi ;
Wen, Zhenhai .
CHINESE JOURNAL OF CATALYSIS, 2020, 41 (05) :858-867
[7]   Unraveling the Origin of Sulfur-Doped Fe-N-C Single-Atom Catalyst for Enhanced Oxygen Reduction Activity: Effect of Iron Spin-State Tuning [J].
Chen, Zhaoyang ;
Niu, Huan ;
Ding, Jie ;
Liu, Heng ;
Chen, Pei-Hsuan ;
Lu, Yi-Hsuan ;
Lu, Ying-Rui ;
Zuo, Wenbin ;
Han, Lei ;
Guo, Yuzheng ;
Hung, Sung-Fu ;
Zhai, Yueming .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2021, 60 (48) :25404-25410
[8]   Applications of M/N/C analogue catalysts in PEM fuel cells and metal-air/oxygen batteries: Status quo, challenges and perspectives [J].
Chi, Bin ;
Zhang, Xiaorong ;
Liu, Mingrui ;
Jiang, Shijie ;
Liao, Shijun .
PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL, 2020, 30 (06) :807-814
[9]   Well-Defined ZIF-Derived Fe-N Codoped Carbon Nanoframes as Efficient Oxygen Reduction Catalysts [J].
Deng, Yijie ;
Dong, Yuanyuan ;
Wang, Guanghua ;
Sun, Kailing ;
Shi, Xiudong ;
Zheng, Long ;
Li, Xiuhua ;
Liao, Shijun .
ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (11) :9699-9709
[10]   A green, cheap, high-performance carbonaceous catalyst derived from Chlorella pyrenoidosa for oxygen reduction reaction in microbial fuel cells [J].
Fan, Zeyu ;
Li, Jun ;
Zhou, Yi ;
Fu, Qian ;
Yang, Wei ;
Zhu, Xun ;
Liao, Qiang .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (45) :27657-27665
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