Hydrogen-rich syngas generation through microwave plasma reforming of greenhouse gases

被引：10

作者：

Akande, Olugbenga ^{[1
,3
,4
]}

Lee, Bongju ^{[3
,4
]}

Okolie, Jude A. ^{[2
]}

Museba, Hugues Nkomba ^{[1
]}

机构：

[1] Handong Global Univ, Dept Comp Sci & Elect Engn, 558 Handong Ro, Pohang 37554, Gyeongsangbuk D, South Korea

[2] Univ Oklahoma, Gallogly Coll Engn, Norman, OK USA

[3] Green Sci Corp, 62 Gyesan 11 Gil, Taebaek Si 26050, Gangwon Do, South Korea

[4] Handong Global Univ, Dept Adv Convergence, 558 Handong Ro, Pohang 37554, Gyeongsangbuk D, South Korea

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2023年 / 48卷 / 89期

关键词：

Noncatalytic greenhouse gas; reforming; Microwave plasma torch; Hydrogen generation; METHANE; ENERGY; FUEL;

D O I：

10.1016/j.ijhydene.2023.05.262

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

This study examined the effectiveness of a 915 MHz atmospheric pressure microwave torch for bulk syngas or hydrogen generation via noncatalytic greenhouse gas (GHG) reforming and its flexibility regarding the amount of soot formed by the process. The investigation shows that plasma-GHG reforming for mass hydrogen generation is feasible without a catalyst at high gas flow rate and microwave power. The best hydrogen production rate and energy yield were 1672 g (H2)/h and 41.8 g (H2)/ kWh, respectively, at 160 lpm gas flow rate and 40 kW microwave power at a CH4/CO2 ratio of 1. The conversion rates of CH4 and CO2 under the same conditions were 95.59% and 95.59%, respectively. The plasma reforming method employed in this study shows its excellent potential for industrial application. (c) 2023 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved

引用

页码：34649 / 34658

页数：10

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