Multifunctional, superelastic, and environmentally stable sodium alginate/mxene/polydimethylsiloxane aerogels for piezoresistive sensor

被引:47
作者
Han, Songjiu [1 ,2 ]
Wu, Qirui [1 ,2 ]
Zhu, Jundong [1 ]
Zhang, Jiayu [1 ]
Chen, Anbang [1 ]
Chen, Yujia [1 ,3 ]
Yang, Xiaoxiang [2 ]
Huang, Jianren [1 ,2 ]
Guan, Lunhui [1 ,3 ]
机构
[1] Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fujian Key Lab Nanomat, Fuzhou 350108, Peoples R China
[2] Fuzhou Univ, Sch Mech Engn & Automat, Fuzhou 350108, Peoples R China
[3] Fuzhou Univ, Sch Chem, Fuzhou 350108, Peoples R China
基金
中国国家自然科学基金;
关键词
MXene aerogel; Piezoresistive sensor; Reversible compression; Environmentally stable; GRAPHENE AEROGELS; CARBON NANOTUBES; STRAIN SENSOR; DISPERSION;
D O I
10.1016/j.cej.2023.144551
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Aerogel sensors have drawn considerable interest in the recent research world. However, simultaneously maintaining superelasticity and an outstanding piezoresistive effect under changing environmental conditions remains challenging. Here, sodium alginate (SA) was used as a bonding agent for MXene nanosheets and polydimethylsiloxane (PDMS) as a reinforcing agent to prepare SA/MXene/PDMS (SMP) composite aerogel with excellent high conductivity, mechanical elasticity, reliable thermal insulation, and good hydrophobicity. The interaction between MXene nanosheets and SA enhances the 3D network framework of the aerogel. The aerogel with a layer-support network structure prepared by the modified directional freezing method showed light weight, high sensitivity (37.43 kPa � 1), significant reversible compression (70%) and excellent fatigue resistance (60,000 cycles). The piezoresistive sensor based on SMP composite aerogel can quickly respond to pressure/ strain signals, which can be further used for pulse beating, sound detection, motion monitoring, foot posture diagnosis and human health monitoring. Additionally, the MXene aerogel sensor based on carbon material with frequency response characteristics can detect low to high frequency vibration signals, has frequency response characteristics that can detect low to high-frequency vibration signals, making it useful for rotating machinery speed detection, cantilever beam vibration detection, non-destructive testing of cantilever beams, and other engineering applications. With its the layered porous structure and the assistance of PDMS, the aerogel also exhibits larger water contact angles (119 degrees) and extreme environmental suitability (-40 to 80 degrees C), performing a wide range of application potential in many fields.
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页数:11
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