Eco-friendly perovskite solar cells: From materials design to device processing and recycling

被引:31
作者
Wu, Xin [1 ]
Zhang, Dong [1 ]
Wang, Xue [1 ]
Jiang, Xiaofen [1 ]
Liu, Baoze [1 ]
Li, Bo [1 ]
Li, Zhen [1 ]
Gao, Danpeng [1 ]
Zhang, Chunlei [1 ]
Wang, Yan [1 ]
Zhu, Zonglong [1 ,2 ,3 ,4 ]
机构
[1] City Univ Hong Kong, Dept Chem, Dept Mat Sci & Engn, Hong Kong, Peoples R China
[2] City Univ Hong Kong, Hong Kong Inst Clean Energy, Hong Kong, Peoples R China
[3] City Univ Hong Kong, Shenzhen Res Inst, Shenzhen, Peoples R China
[4] City Univ Hong Kong, Dept Chem, Dept Mat Sci & Engn, Hong Kong 999077, Peoples R China
关键词
eco-friendly; green solvent; lead adsorbent; lead-free; perovskite solar cells; PHOTOVOLTAIC PERFORMANCE; SURFACE PASSIVATION; HIGHLY EFFICIENT; LEAD; STABILITY; FILMS; FABRICATION; CS2AGBIBR6; DEFECTS; STEP;
D O I
10.1002/eom2.12352
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
With the skyrocketed power conversion efficiency and enhanced lifetime of perovskite solar cells (PVSCs), the environmental issues from materials to device processing, operation, and recycling become critical for their commercialization. Developing eco-friendly PVSCs via the exploration of lead-free perovskite materials, non-toxic solvents, and effective lead-adsorbing materials are the key points to realizing eco-friendly PVSCs, which have drawn significant attention in the past 3 years. This critical review presents a comprehensive overview of the recent progress of eco-friendly PVSCs in a close loop, including eco-friendly perovskite materials, eco-friendly device processing, eco-friendly device operation, and eco-friendly perovskite recycling. The innovation of perovskite materials, criteria of green solvent selection, and design principles of lead adsorbents are thoroughly introduced, with their combination for the device processing and operation well explained. An outlook of further material innovation and device optimization is provided to offer instruction for the development of this research field.
引用
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页数:18
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