Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy

被引:3
|
作者
Liang, Shuang [1 ,2 ]
Biesold, Gill M. M. [1 ]
Zhuang, Mingyue [1 ,4 ]
Kang, Zhitao [3 ]
Wagner, Brent [3 ]
Lin, Zhiqun [1 ,4 ]
机构
[1] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA
[2] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
[3] Georgia Inst Technol, Georgia Tech Res Inst, Atlanta, GA 30332 USA
[4] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore
来源
NANOSCALE ADVANCES | 2023年 / 5卷 / 07期
基金
美国国家科学基金会;
关键词
MICROFLUIDIC PLATFORM; BRIGHTLY LUMINESCENT; DEFECT-TOLERANCE; CH3NH3PBX3; X; SOLAR-CELLS; FLOW; BR; STABILITY; CL; PHOTOSTABILITY;
D O I
10.1039/d2na00744d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Lead halide perovskite nanocrystals possess incredible potential as next generation emitters due to their stellar set of optoelectronic properties. Unfortunately, their instability towards many ambient conditions and reliance on batch processing hinder their widespread utilities. Herein, we address both challenges by continuously synthesizing highly stable perovskite nanocrystals via integrating star-like block copolymer nanoreactors into a house-built flow reactor. Perovskite nanocrystals manufactured in this strategy display significantly enhanced colloidal, UV, and thermal stabilities over those synthesized with conventional ligands. Such scaling up of highly stable perovskite nanocrystals represents an important step towards their eventual use in many practical applications in optoelectronic materials and devices.
引用
收藏
页码:2038 / 2044
页数:7
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