Advances in photothermal conversion of carbon dioxide to solar fuels

被引:31
作者
Gao, Wa [1 ]
Li, Yinwen [2 ,3 ]
Xiao, Dequan [4 ]
Ma, Ding [2 ,3 ]
机构
[1] Beijing Univ Agr, Coll Biosci & Resources Environm, Beijing 102206, Peoples R China
[2] Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China
[3] Peking Univ, Coll Engn, Beijing 100871, Peoples R China
[4] Univ New Haven, Ctr Integrat Mat Discovery, Dept Chem & Chem & Biomed Engn, West Haven, CT 06516 USA
来源
JOURNAL OF ENERGY CHEMISTRY | 2023年 / 83卷
关键词
Solar energy; Photothermal catalysis; CO2; reduction; Catalyst design; Performance improvement; SURFACE-PLASMON RESONANCE; VISIBLE-LIGHT IRRADIATION; CATALYTIC CO2 CONVERSION; PHOTOCATALYTIC REDUCTION; PT/TIO2; PHOTOCATALYSTS; GOLD NANOPARTICLES; ROOM-TEMPERATURE; CHARGE-TRANSFER; DRIVEN; ENERGY;
D O I
10.1016/j.jechem.2023.04.024
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
Converting carbon dioxide (CO2) into useful fuels or chemical feedstocks is important for achieving peak carbon emission and carbon neutrality. Recently, photothermal catalysis has been extensively studied and applied due to its advantages over traditional heat-driven catalysis. In this review, we focus on photothermal catalysis of thermodynamically uphill reactions that convert CO2 into value-added products. We first introduce the fundamentals of photothermal catalysis for CO2 reduction, including the definition and classification of photothermal catalysis, followed by their photothermal conversion processes. The structure design of different types of photothermal catalysts is summarized. The superior performance of photothermal catalytic conversion of CO2 is illustrated and discussed, including improved CO2 activation, tunable selectivity towards different solar fuel products, and resistance to sintering and coking. Finally, the perspectives and challenges in this cutting-edge field are presented with the aim of advancing understanding of the underlying mechanisms and inspiring rational design of photothermal catalysts for highly efficient solar-to-fuel conversion. (c) 2023 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press.
引用
收藏
页码:62 / 78
页数:17
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